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Quantum critical behavior of the hyperkagome magnet <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mi mathvariant="normal">Mn</mml:mi><mml:mn>3</mml:mn></mml:msub><mml:mi>CoSi</mml:mi></mml:math>

2024· article· lv· W4391530763 on OpenAlexafffund
Hiroki Yamauchi, Dita Puspita Sari, Yukio Yasui, Terutoshi Sakakura, Hiroyuki Kimura, Akiko Nakao, Takashi Ohhara, T. Honda, Katsuaki Kodama, Naoki Igawa, Kazutaka Ikeda, Kazuki Iida, Daichi Ueta, Tetsuya Yokoo, Matthias Frontzek, Songxue Chi, J. A. Fernandez‐Baca, Kenji Kojima, Donald J. Arseneau, G. D. Morris, B. Hitti, Yipeng Cai, Adam Berlie, Isao Watanabe, Pai-Tse Hsu, Yu‐Sheng Chen, Min Kai Lee, A. E. Hall, G. Balakrishnan, L. J. Chang, Shin‐ichi Shamoto

Bibliographic record

VenuePhysical Review Research · 2024
Typearticle
Languagelv
FieldMaterials Science
TopicMagnetic and transport properties of perovskites and related materials
Canadian institutionsTRIUMF
FundersOak Ridge National LaboratoryNational Science and Technology CouncilBasic Energy SciencesJapan Atomic Energy AgencyJapan Society for the Promotion of ScienceNational Cheng Kung UniversityUniversity of TokyoEngineering and Physical Sciences Research CouncilTRIUMFUnited States-Japan FoundationU.S. Department of EnergyUniversity of Warwick
KeywordsPhysics

Abstract

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<a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:mi>β</a:mi></a:math>-Mn-type family alloys <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"><b:mrow><b:msub><b:mi>Mn</b:mi><b:mn>3</b:mn></b:msub><b:mrow><b:mi>T</b:mi><b:mi>X</b:mi></b:mrow></b:mrow></b:math> (<c:math xmlns:c="http://www.w3.org/1998/Math/MathML"><c:mrow><c:mi>T</c:mi><c:mo>=</c:mo><c:mtext>Co</c:mtext></c:mrow></c:math>, Rh, and Ir; <d:math xmlns:d="http://www.w3.org/1998/Math/MathML"><d:mrow><d:mi>X</d:mi><d:mo>=</d:mo><d:mtext>Si</d:mtext></d:mrow></d:math> and Ge) have a three-dimensional antiferromagnetic (AF) corner-shared triangular network, i.e., the hyperkagome lattice. The antiferromagnet <e:math xmlns:e="http://www.w3.org/1998/Math/MathML"><e:mrow><e:msub><e:mi>Mn</e:mi><e:mn>3</e:mn></e:msub><e:mi>RhSi</e:mi></e:mrow></e:math> shows magnetic short-range order over a wide temperature range of approximately 500 K above the Néel temperature <f:math xmlns:f="http://www.w3.org/1998/Math/MathML"><f:msub><f:mi>T</f:mi><f:mi mathvariant="normal">N</f:mi></f:msub></f:math> of 190 K. In this family of compounds, as the lattice parameter decreases, the long-range magnetic ordering temperature decreases. <h:math xmlns:h="http://www.w3.org/1998/Math/MathML"><h:mrow><h:msub><h:mi>Mn</h:mi><h:mn>3</h:mn></h:msub><h:mi>CoSi</h:mi></h:mrow></h:math> has the smallest lattice parameter and the lowest <i:math xmlns:i="http://www.w3.org/1998/Math/MathML"><i:msub><i:mi>T</i:mi><i:mi mathvariant="normal">N</i:mi></i:msub></i:math> in the family. The quantum critical point (QCP) from AF to the quantum paramagnetic state is expected near a cubic lattice parameter of 6.15 <k:math xmlns:k="http://www.w3.org/1998/Math/MathML"><k:mi>Å</k:mi></k:math>. Although the Néel temperature of <l:math xmlns:l="http://www.w3.org/1998/Math/MathML"><l:mrow><l:msub><l:mi>Mn</l:mi><l:mn>3</l:mn></l:msub><l:mi>CoSi</l:mi></l:mrow></l:math> is only 140 K, the emergence of the quantum critical behavior in <m:math xmlns:m="http://www.w3.org/1998/Math/MathML"><m:mrow><m:msub><m:mi>Mn</m:mi><m:mn>3</m:mn></m:msub><m:mi>CoSi</m:mi></m:mrow></m:math> is discussed. We study how the magnetic short-range order appears in <n:math xmlns:n="http://www.w3.org/1998/Math/MathML"><n:mrow><n:msub><n:mi>Mn</n:mi><n:mn>3</n:mn></n:msub><n:mi>CoSi</n:mi></n:mrow></n:math> by using neutron scattering, <o:math xmlns:o="http://www.w3.org/1998/Math/MathML"><o:mrow><o:mi>μ</o:mi><o:mi>SR</o:mi></o:mrow></o:math>, and bulk characterization such as specific heat capacity. According to the results, the neutron scattering intensity of the magnetic short-range order in <p:math xmlns:p="http://www.w3.org/1998/Math/MathML"><p:mrow><p:msub><p:mi>Mn</p:mi><p:mn>3</p:mn></p:msub><p:mi>CoSi</p:mi></p:mrow></p:math> does not change much at low temperatures from that of <q:math xmlns:q="http://www.w3.org/1998/Math/MathML"><q:mrow><q:msub><q:mi>Mn</q:mi><q:mn>3</q:mn></q:msub><q:mi>RhSi</q:mi></q:mrow></q:math>, although the <r:math xmlns:r="http://www.w3.org/1998/Math/MathML"><r:mrow><r:mi>μ</r:mi><r:mi>SR</r:mi></r:mrow></r:math> short-range order temperature of <s:math xmlns:s="http://www.w3.org/1998/Math/MathML"><s:mrow><s:msub><s:mi>Mn</s:mi><s:mn>3</s:mn></s:msub><s:mi>CoSi</s:mi></s:mrow></s:math> is largely suppressed to 240 K from that of <t:math xmlns:t="http://www.w3.org/1998/Math/MathML"><t:mrow><t:msub><t:mi>Mn</t:mi><t:mn>3</t:mn></t:msub><t:mi>RhSi</t:mi></t:mrow></t:math>. Correspondingly, the volume fraction of the magnetic short-range order regions, as shown by the initial asymmetry drop ratio of <u:math xmlns:u="http://www.w3.org/1998/Math/MathML"><u:mrow><u:mi>μ</u:mi><u:mi>SR</u:mi></u:mrow></u:math> above <v:math xmlns:v="http://www.w3.org/1998/Math/MathML"><v:msub><v:mi>T</v:mi><v:mi mathvariant="normal">N</v:mi></v:msub></v:math>, also becomes small. Instead, the electronic-specific heat coefficient <x:math xmlns:x="http://www.w3.org/1998/Math/MathML"><x:mi>γ</x:mi></x:math> of <y:math xmlns:y="http://www.w3.org/1998/Math/MathML"><y:mrow><y:msub><y:mi>Mn</y:mi><y:mn>3</y:mn></y:msub><y:mi>CoSi</y:mi></y:mrow></y:math> is the largest in this <z:math xmlns:z="http://www.w3.org/1998/Math/MathML"><z:mrow><z:msub><z:mi>Mn</z:mi><z:mn>3</z:mn></z:msub><z:mi>T</z:mi><z:mi>Si</z:mi></z:mrow></z:math> system, possibly due to the low-energy spin fluctuation near the quantum critical point. Published by the American Physical Society 2024

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.004
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Scholarly communication, Insufficient payload (model declined to judge)
Consensus categoriesScience and technology studies, Insufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.885
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0040.002
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.001
Science and technology studies0.0010.003
Scholarly communication0.0010.001
Open science0.0020.002
Research integrity0.0010.002
Insufficient payload (model declined to judge)0.1340.006

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.039
GPT teacher head0.307
Teacher spread0.268 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations6
Published2024
Admission routes2
Has abstractyes

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