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Record W4392236914 · doi:10.1002/cjce.25218

Experimental methods in chemical engineering: X‐ray fluorescence— <scp>XRF</scp>

2024· article· en· W4392236914 on OpenAlexaffvenue
Mario Ferreiro González, Nooshin Saadatkhah, Gregory S. Patience

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2024
Typearticle
Languageen
FieldPhysics and Astronomy
TopicX-ray Spectroscopy and Fluorescence Analysis
Canadian institutionsPolytechnique Montréal
Fundersnot available
KeywordsX-ray fluorescenceFluorescenceElectronRange (aeronautics)Analytical Chemistry (journal)Atomic orbitalChemistryMaterials scienceNanotechnologyAtomic physicsPhysicsNuclear physicsOpticsEnvironmental chemistryComposite material

Abstract

fetched live from OpenAlex

Abstract X‐ray fluorescence (XRF) is a non‐destructive spectrometric technique to detect elements with an atomic number from 11 (sodium) and beyond 92 (uranium). When X‐rays or gamma rays eject tightly bound inner core electrons, an electron from an outer shell will fill the empty orbital and fluoresce. Every element has a characteristic fluorescence, which depends on the element and the electrons in the orbitals that are ejected and those that fill the orbital. With the characteristic energy of the fluorescence, we determine elemental composition and concentration when adequately calibrated. Typical run times range from a second to a few minutes with an sensitivity to as low as (ppm). XRF guns are portable devices that produce qualitative data while libraries loaded to laboratory instruments are capable of producing quantitative data. A broad range of scientists and engineers apply XRF in research—140 of the 250 scientific categories in the Web of Science (WoS) cite XRF analyses. Of the 10,000 articles indexed in WoS since 2018, chemical engineering ranks fifth with the most articles. The focus of the research in this category includes adsorption and waste water, combustion and pyrolysis, catalysis and zeolites, and nanoparticles and oxidation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.003
metaresearch head score (Gemma)0.003
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Methods · Consensus signal: Methods
Teacher disagreement score0.022
Threshold uncertainty score0.074

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0030.003
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0030.003
Science and technology studies0.0020.002
Scholarly communication0.0020.002
Open science0.0020.002
Research integrity0.0020.002
Insufficient payload (model declined to judge)0.0220.016

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.258
Teacher spread0.250 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations24
Published2024
Admission routes2
Has abstractyes

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