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Record W4392501585 · doi:10.1088/2053-1591/ad30a8

Enhanced high-temperature tribological performance of fluorinated tetrahedral amorphous carbon (ta-C:F) coatings in sliding applications

2024· article· en· W4392501585 on OpenAlex
S. Bhowmick, Shayan Shirzadian, A.T. Alpas

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueMaterials Research Express · 2024
Typearticle
Languageen
FieldMaterials Science
TopicDiamond and Carbon-based Materials Research
Canadian institutionsUniversity of Windsor
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsMaterials scienceTribologyRaman spectroscopyAmorphous solidAmorphous carbonX-ray photoelectron spectroscopyFluorineCarbon fibersDissolutionContact angleComposite materialMetallurgyChemical engineeringCrystallographyChemistryComposite number

Abstract

fetched live from OpenAlex

Abstract This study investigated the dry sliding behaviour of fluorinated tetrahedral amorphous carbon (ta-C:F) coatings against uncoated 52100 steel at temperatures ranging from 25 °C to 300 °C. The ta-C:F coatings demonstrated significant reductions in both the coefficient of friction(COF) during the running-in stage and at steady state, particularly within the temperature range of 25 °C to 200 °C, surpassing the performance of well-established a-C:H coatings. SEM analyses revealed the formation of transfer layers on the contact surface of 52100 steel when tested against ta-C:F coatings at temperatures up to 200 °C, while none were detected at temperatures ≥250 °C. Raman spectroscopy indicated a transition from sp 3 to sp 2 carbon structures in the carbonaceous transfer layers with increasing temperature, and XPS scans confirmed an increase in fluorine (F) concentration within these layers, correlating with reduced COF. The comparative analysis at 120 °C emphasized the intrinsic advantages of ta-C:F coatings in high-temperature applications, demonstrating a nearly 50% lower COF (0.08) when compared to traditional boundary-lubricated steel-to-steel sliding contacts. These findings have significant implications for enhancing the efficiency and durability of various mechanical systems, particularly in industries like automotive and manufacturing.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.004
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0040.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.030
GPT teacher head0.324
Teacher spread0.294 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it