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Record W4392650882 · doi:10.5194/egusphere-egu24-21098

Impact of using a 3.5 μm film to analyze the chemical composition of crystal samples with a handheld X-Ray Fluorescence equipment

2024· preprint· en· W4392650882 on OpenAlexaff
Filipa Dias, Ricardo Ribeiro, Alexandre Lima, Filipe Gonçalves, Encarnación Roda-Robles, Tânia Martins

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldPhysics and Astronomy
TopicX-ray Spectroscopy and Fluorescence Analysis
Canadian institutionsManitoba Hydro
Fundersnot available
KeywordsMobile deviceComposition (language)X-rayFluorescenceX-ray fluorescenceMaterials scienceAnalytical Chemistry (journal)Crystal (programming language)ChemistryComputer scienceOpticsPhysicsChromatographyWorld Wide WebArt

Abstract

fetched live from OpenAlex

Some potassium-feldspar crystals from lithium-rich aplite-pegmatites from Northern Portugal have been analyzed with a handheld X-Ray-Fluorescence (XRF) equipment. This study compares the impact of analyzing the samples with an XRF film versus analyzing them without it. The film used was a Hitachi Poly-S High Performance XRF Sample Film of 3.5 μm, commonly used for analyzing samples in cups and powders. Although Hitachi alerts for the unsuitability of the film for analyzing light elements, this study helps understand the extent of error that this film can cause when analyzing this type of sample. 15 cleaned potassium feldspar crystals with a size between 1-3 cm have been analyzed with a Bruker S1 TITAN 600 containing an X-ray tube with a 2 W and 5-100 μA Rh anode. The Geomining factory calibration was used for the sample analysis.The results show that the potassium-feldspars analyzed with the film had their major elements drop by 20-40% for silica (SiO2), 30-50% for aluminum (Al2O3) and 10-20% for potassium (K2O). As for the trace elements, calcium (Ca) dropped by 20-30%, phosphorous (P) by 20-40% and rubidium (Rb) and iron (Fe) have small errors that can vary from plus 0-10% to minus 0-10%. Knowing the film impact will hopefully be of assistance for the correct interpretation of portable XRF results during field campaigns for mineral exploration.This study was financially supported by FCT, I.P., in the framework of the ICT (UIDB/04683/2020 and UIDP/04683/2020), by the PhD project (2020.05534.BD) and by national funds from MCTES, through FCT, co-financed by ESF through POCH and NORTE 2020. This work is also supported by the Greenpeg project, reference 869274, funded by the Horizon 2020 framework program of the European Union.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.117
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.309
Teacher spread0.288 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes1
Has abstractyes

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