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Record W4392760066 · doi:10.5194/egusphere-egu24-13836

Consumption of methane by a landfill cover soil under variable moisture and temperature conditions

2024· preprint· en· W4392760066 on OpenAlexaffabout
Christina Lam, Stephanie Slowinski, Mehdi Ramezanzadeh, Laura Hug, Nathanael Willms, Philippe Van Cappellen, Fereidoun Rezanezhad

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldEnvironmental Science
TopicLandfill Environmental Impact Studies
Canadian institutionsUniversity of Waterloo
Fundersnot available
KeywordsMethaneCover (algebra)Environmental scienceMoistureWater contentVariable (mathematics)Soil coverSoil scienceMathematicsGeologyChemistryGeotechnical engineeringGeographySoil waterEngineeringMeteorology

Abstract

fetched live from OpenAlex

Landfills are one of the largest anthropogenic sources of methane (CH4), and hot-spots of CH4 emissions in landfill cover soils can enrich microbes that oxidize CH4 to carbon dioxide (CO2). CH4 oxidation rates are modulated by multiple variables including soil moisture and temperature, although the interactive effects of these factors on CH4 oxidation rates have not been well-studied. Here, we conducted a closed-headspace batch experiment with cover soil from a former landfill in Ontario, Canada to measure CH4 consumption and CO2 efflux rates associated with variations in soil moisture and temperature simultaneously. Soil samples were incubated under a factorial design of 5 soil moisture contents ranging from 11 to 47% WFPS (water-filled pore space), and 6 temperatures ranging from 1 to 35°C. At each temperature and WFPS combination, CH4 (812 nmol) was spiked into the headspace, and headspace CH4 and CO2 concentrations were measured over 2 hours to calculate CO2 efflux and CH4 consumption rates. The maximum CO2 efflux rate was observed at the maximal WFPS and temperature conditions of this experiment (92 nmol h-1 g dry wt.-1 at 47% WFPS and 35°C), while the maximum CH4 consumption rate was observed at intermediate WFPS and temperature conditions (1.9 nmol h-1 g dry wt.-1 at 25% WFPS and 25°C). The CO2 efflux observed is primarily attributed to the oxidative degradation of soil organic matter. A diffusion-reaction model was fit to the observed data to represent the effects of temperature and soil WFPS on the CH4 consumption and CO2 efflux rates. The model predicted similar optimal conditions as those observed for both the CH4 consumption and the CO2 efflux rates. The modeling and experimental results show that the dominant controls on optimal soil moisture for CH4 consumption are moisture limitation of microbial activity and of gas (CH4 and oxygen) diffusion, versus the interactive effects of moisture limitation of gas (oxygen) diffusion and of solute mobility for CO2 effluxes. These results provide insight into how seasonal changes in soil moisture and temperature could impact CH4 oxidation rates, and therefore also net CH4 emissions, in landfill cover soils and other environments.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.149
Threshold uncertainty score0.296

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.245
Teacher spread0.235 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes2
Has abstractyes

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