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Record W4392993860 · doi:10.1021/acs.iecr.3c04671

Separation of Magnesium Impurity from Nickel and Cobalt Mixtures Using Ethylenediaminetetraacetic Acid and Temperature Optimization

2024· article· en· W4392993860 on OpenAlex
Hongting Liu, Monu Malik, Kyoung Hun Choi, Gisele Azimi

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2024
Typearticle
Languageen
FieldEngineering
TopicExtraction and Separation Processes
Canadian institutionsUniversity of Toronto
FundersHatchNatural Sciences and Engineering Research Council of Canada
KeywordsEthylenediaminetetraacetic acidCobaltImpurityMagnesiumNickelInorganic chemistryChemistryMaterials scienceChelationMetallurgyOrganic chemistry

Abstract

fetched live from OpenAlex

This study aims to develop a process for separating magnesium from nickel and cobalt pregnant leach solutions, overcoming the limitations of conventional metal separation techniques. The process utilizes ethylenediaminetetraacetic acid (EDTA) for complexation, selectively binding with nickel and cobalt to reduce their coprecipitation with magnesium. Thermodynamic simulations and kinetic experiments are conducted at varying temperatures (25, 50, and 75 °C) to optimize the complexation and separation efficiency. The research demonstrates that increasing the temperature significantly accelerates the complexation kinetics, reducing the required time to less than 1 h. At 75 °C, over 98% of magnesium was selectively removed with minimal coprecipitation of nickel and cobalt (less than 2%). The study also highlights the reusability of EDTA, enhancing the process’s economic and environmental viability. The developed process offers a rapid alternative to conventional methods for separating magnesium from nickel and cobalt mixtures. This method has potential applications in other industrial processes, particularly in hydrometallurgy, where rapid and selective metal separation is crucial. Further research is suggested to refine the process for specific industrial applications, focusing on scalability, cost-effectiveness, and environmental aspects. The adaptability of the method to other metal systems also presents an exciting avenue for future exploration in the metal processing industries.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.244
Threshold uncertainty score0.655

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.050
GPT teacher head0.335
Teacher spread0.285 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it