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Record W4393043371 · doi:10.1016/j.jcou.2024.102736

Carbon dioxide sequestration through steel slag carbonation: Review of mechanisms, process parameters, and cleaner upcycling pathways

2024· article· en· W4393043371 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueJournal of CO2 Utilization · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicCO2 Sequestration and Geologic Interactions
Canadian institutionsMcMaster UniversityNatural Resources Canada
FundersOffice of Energy Research and DevelopmentMcMaster University
KeywordsCarbonationCarbon sequestrationSlag (welding)SteelmakingEnvironmental scienceWaste managementCarbon dioxideProcess (computing)Cleaner productionProcess engineeringMaterials scienceMetallurgyEngineeringMunicipal solid wasteChemistryComputer scienceComposite material

Abstract

fetched live from OpenAlex

The direct carbonation of steel slag has emerged as a promising approach for carbon dioxide (CO2) utilization and sequestration, holding potential for advancing sustainable steel production. Despite considerably high expectations for these cleaner upcycling pathways, their maturity level remains relatively low and large-scale direct carbonation of steel slag is largely untested. To facilitate steel slag carbonation on a scale necessary for a zero-carbon future economy, this article provides a comprehensive review of fundamental carbonation mechanisms and critical parameters governing the reaction process, including temperature, pressure, reaction time, liquid-to-solid ratio, and CO2 partial pressure. The study critically examines the unique interactions among these process parameters, which can either limit or enhance the process optimization. The spectrum of scientific challenges associated with this pathway, including reaction rate limitations and the carbonated product valorization, particularly as a binder or aggregate in the construction sector, are identified and addressed. These insights aim to enhance the carbonation potential of steel slag for possible cleaner upcycling implementation pathways, ultimately facilitating the development of more efficient and sustainable carbon capture utilization and sequestration (CCUS) technologies. The proposed improvements are expected to be instrumental in promoting sustainable practices, not only to foster the decarbonization of the steelmaking industry but also in aiding other hard-to-abate sectors, such as the cement and concrete industry, in achieving their own decarbonization goals.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.220
Threshold uncertainty score0.335

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.046
GPT teacher head0.309
Teacher spread0.263 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it