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Record W4393232877 · doi:10.1039/bk9781837672035-00106

Chemical transformations using GaN-based catalysts

2024· book-chapter· en· W4393232877 on OpenAlexaff
Jing‐Tan Han, Lida Tan, Hui Su, Chao‐Jun Li

Bibliographic record

Venuenot available
Typebook-chapter
Languageen
FieldChemical Engineering
TopicAmmonia Synthesis and Nitrogen Reduction
Canadian institutionsMcGill UniversityCentre in Green Chemistry and Catalysis
Fundersnot available
KeywordsCatalysisMaterials scienceChemical engineeringChemistryEngineeringOrganic chemistry

Abstract

fetched live from OpenAlex

Gallium nitride (GaN), a wide bandgap III–V semiconductor, has been extensively applied in lighting, electronics, and radiofrequency devices over the last few decades. With the distinct properties of fast charge mobility, high stability, tunable wide bandgap, and ionicity structure, GaN-based catalysts have drawn considerable attention in chemical synthesis recently. In this chapter, the recent progress and critical breakthrough of GaN-based catalysis in synthesis are reviewed, with a focus on mechanistic understanding. The reactions are categorized as water splitting, direct methane activation, direct methanol activation, organic synthesis, carbon dioxide reduction, and nitrogen gas reduction. Lastly, the challenges and future possible improvement of GaN-based catalysis are discussed, to encourage more interdisciplinary advances in the development of novel catalysts for sustainable chemical transformations.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Other · Consensus signal: Other
Teacher disagreement score0.434
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.231
Teacher spread0.209 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes1
Has abstractyes

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