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Record W4393319606 · doi:10.1021/acssusresmgt.3c00052

Integration of Electrochemical Oxidation and Photocatalytic Degradation with Robust Synergistic Effect for Efficient Wastewater Treatment

2024· article· en· W4393319606 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueACS Sustainable Resource Management · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicWater Quality Monitoring and Analysis
Canadian institutionsUniversity of GuelphLakehead University
FundersNatural Sciences and Engineering Research Council of CanadaCanada Foundation for Innovation
KeywordsPhotocatalysisDegradation (telecommunications)ElectrochemistryWastewaterSewage treatmentChemistryChemical engineeringEnvironmental scienceMaterials scienceEnvironmental chemistryCatalysisComputer scienceEnvironmental engineeringElectrodeEngineeringOrganic chemistryTelecommunications

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide In this study, a novel design of an integrated electrode is introduced for the photoelectrochemical purification of water from a wastewater treatment plant. A nanoporous TiO 2 structure, directly grown on a Ti substrate by anodization, and a RuO 2 –IrO 2 -based electrode were utilized as the photocatalyst and the electrocatalyst, respectively. Photocatalytic and electrocatalytic activities were synergistically combined to achieve an integrated and highly catalytically active electrode. This design, wherein there was no surface contact between the photocatalyst and the electrocatalyst, significantly minimized the chance of electron–hole recombination. The experimental results have shown that the efficient enablement of photocatalytic and electrocatalytic activities within a single integrated electrode may be achieved via this design. The applicability of this integrated electrode system was also tested in a pilot plant with a capacity to hold 40 L of water at a water treatment facility. The pilot plant testing results revealed that ca. 75% removal of organic waste was accomplished using the integrated electrode system compared to only photocatalyst (∼20%) or electrocatalyst (∼40%). The innovative strategy demonstrated in the present study may facilitate various combinations of electrocatalysts and photocatalysts, and its scalability renders it adaptable to the different industrial requirements with ease.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.161
Threshold uncertainty score0.414

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.223
Teacher spread0.215 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it