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Record W4394570478 · doi:10.1038/s41467-024-47291-8

Nonlinear optical diode effect in a magnetic Weyl semimetal

2024· article· en· W4394570478 on OpenAlexafffund
Christian Tzschaschel, Jian-Xiang Qiu, Xue-Jian Gao, H. Li, Chunyu Guo, Hung‐Yu Yang, Cheng-Ping Zhang, Ying-Ming Xie, Yufei Liu, Anyuan Gao, Damien Bérubé, Thao Dinh, Sheng-Chin Ho, Yuqiang Fang, Fuqiang Huang, Johanna Nordlander, Qiong Ma, Fazel Tafti, Philip J. W. Moll, K. T. Law, Su‐Yang Xu

Bibliographic record

VenueNature Communications · 2024
Typearticle
Languageen
FieldPhysics and Astronomy
TopicTopological Materials and Phenomena
Canadian institutionsCanadian Institute for Advanced Research
FundersAir Force Office of Scientific ResearchDivision of Materials ResearchOffice of ScienceEuropean CommissionSchweizerischer Nationalfonds zur Förderung der Wissenschaftlichen ForschungU.S. Department of DefenseU.S. Department of EnergyCanadian Institute for Advanced ResearchNational Natural Science Foundation of ChinaHarvard UniversityNational Science Foundation
KeywordsWeyl semimetalPhysicsMagnetizationDiodeSecond-harmonic generationNode (physics)Condensed matter physicsNonlinear systemNonlinear opticalTopology (electrical circuits)OptoelectronicsSemimetalMagnetic fieldOpticsLaserQuantum mechanicsElectrical engineering

Abstract

fetched live from OpenAlex

Diode effects are of great interest for both fundamental physics and modern technologies. Electrical diode effects (nonreciprocal transport) have been observed in Weyl systems. Optical diode effects arising from the Weyl fermions have been theoretically considered but not probed experimentally. Here, we report the observation of a nonlinear optical diode effect (NODE) in the magnetic Weyl semimetal CeAlSi, where the magnetization introduces a pronounced directionality in the nonlinear optical second-harmonic generation (SHG). We demonstrate a six-fold change of the measured SHG intensity between opposite propagation directions over a bandwidth exceeding 250 meV. Supported by density-functional theory, we establish the linearly dispersive bands emerging from Weyl nodes as the origin of this broadband effect. We further demonstrate current-induced magnetization switching and thus electrical control of the NODE. Our results advance ongoing research to identify novel nonlinear optical/transport phenomena in magnetic topological materials and further opens new pathways for the unidirectional manipulation of light.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Theoretical or conceptual · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.765
Threshold uncertainty score0.551

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.292
Teacher spread0.283 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designTheoretical or conceptual
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations18
Published2024
Admission routes2
Has abstractyes

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