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Record W4394687554 · doi:10.1016/j.biosx.2024.100479

Sensitivity studies and optimization of an impedance-based biosensor for point-of-care applications

2024· article· en· W4394687554 on OpenAlexaff
Tianxiang Jiang, Xuanjie Ye, Zuyuan Tian, Mohamed Shaheen, Ahmed A. Khorshed, Yiwei Feng, Bingxuan Li, Yusheng Zhang, Xihua Wang, Jie Chen

Bibliographic record

VenueBiosensors and Bioelectronics X · 2024
Typearticle
Languageen
FieldChemical Engineering
TopicAnalytical Chemistry and Sensors
Canadian institutionsUniversity of Alberta
FundersChina Scholarship Council
KeywordsSensitivity (control systems)BiosensorPoint of careElectrical impedanceComputer sciencePoint (geometry)Point-of-care testingMaterials scienceBiochemical engineeringBiological systemNanotechnologyElectronic engineeringMedicineBiologyMathematicsEngineeringElectrical engineeringPathology

Abstract

fetched live from OpenAlex

In this study, we examined the relationship between the sensitivity of interdigitated electrode (IDE) impedimetric biosensors and the gap between the IDEs. Our aim is to find an optimal design to maximize sensitivity. A three-dimensional COMSOL model was constructed for determining the effects of electrode gap, width, and height on impedance sensitivity, revealing a singular linear correlation with the inner gap. Considering both the simulation results and fabrication processes, we have developed three IDE prototype chips with electrode gaps of 3 μm, 4 μm, and 5 μm, respectively. For empirical validation, human anti-SARS-CoV-2 monoclonal antibody (mAb) was utilized, with immobilization of the SARS-CoV-2 spike protein on the chip's surface for mAb capture. This interaction, further amplified by Protein G conjugation, induced shifts in the impedance spectrum. The sensitivity of each prototype chip was evaluated across mAb concentrations ranging from 50 ng/mL to 500 ng/mL. The 3 μm configuration emerged as the most sensitive, demonstrating the ability to detect mAb concentrations as low as 50 ng/mL, a threshold unattainable by the other designs. This outcome underscores the critical influence of reduced inter-electrode gap on enhancing biosensor detection limits. The findings from this investigation offer a foundational approach for advancing biosensor sensitivity via electrode geometric optimization, with broad potential applications extending beyond COVID-19 diagnostics to a wide spectrum of clinical and research contexts.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.445
Threshold uncertainty score0.490

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.278
Teacher spread0.264 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2024
Admission routes1
Has abstractyes

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