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Record W4396552700 · doi:10.31031/pps.2024.06.000632

Towards Sustainable Fuels from Fischer-Tropsch Synthesis

2024· article· en· W4396552700 on OpenAlexaff
Zahra Teimouri

Bibliographic record

VenueProgress in Petrochemical Science · 2024
Typearticle
Languageen
FieldChemical Engineering
TopicCatalysts for Methane Reforming
Canadian institutionsMcMaster University
Fundersnot available
KeywordsFischer–Tropsch processChemistryEnvironmental scienceOrganic chemistryCatalysis

Abstract

fetched live from OpenAlex

Fischer-Tropsch Synthesis (FTS) is a non-crude oil-based technique for conversion of syngas to a wide range of hydrocarbons including light olefins, and liquid transportation fuels.Syngas, which is a combination of H 2 and CO gases can be produced through natural gas reforming, biomass or coal gasification processes.FTS is a catalytic polymerization reaction, therefore rational design of the catalyst including active sites, support and promoters plays a significant role in improving the selectivity of the process to desired range of products.This mini review presents a summary of the different catalyst designs in FTS to synthesize light olefins or heavier hydrocarbons.Iron and cobalt are the industrially used active metals for FTS, due to the lower price and higher hydrogenation activity, respectively.Supports are a key factor in designing efficient FTS catalysts, which provide mechanical, thermal strength for the active sites and a high surface area for dispersion of the active metal particles.Herein we discuss two categories of the widely used support material for FTS: metal oxide supports and carbon materials.Another significant element in formulating a high-performance catalyst for FTS process is the promoters, which can be divided into electronical and structural promoters.This work highlights the roles of active metal, support and promoters in understanding the structure-activity correlations to design high-performance FTS catalysts for production clean and sustainable fuels.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.005
Threshold uncertainty score0.016

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0010.001
Scholarly communication0.0010.003
Open science0.0010.002
Research integrity0.0020.003
Insufficient payload (model declined to judge)0.0050.004

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.276
Teacher spread0.266 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes1
Has abstractyes

Explore more

Same venueProgress in Petrochemical ScienceSame topicCatalysts for Methane ReformingFrench-language works237,207