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Record W4399154844 · doi:10.1021/acssusresmgt.3c00025

High Surface Area Microporous Activated Carbon from Corn Fiber Using Graphene Oxide-Assisted Hydrothermal Carbonization

2024· article· en· W4399154844 on OpenAlex
Mitchell Ubene, Kevin MacDermid-Watts, Animesh Dutta, Colin van der Kuur

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueACS Sustainable Resource Management · 2024
Typearticle
Languageen
FieldMaterials Science
TopicGraphene research and applications
Canadian institutionsUniversity of Guelph
FundersNatural Sciences and Engineering Research Council of CanadaOntario Ministry of Agriculture, Food and Rural Affairs
KeywordsCarbonizationMicroporous materialHydrothermal carbonizationMaterials scienceGrapheneHydrothermal circulationOxideChemical engineeringFiberActivated carbonCarbon fibersSpecific surface areaNanotechnologyAdsorptionComposite materialChemistryCatalysisMetallurgyComposite numberOrganic chemistryScanning electron microscope

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide This study investigated a novel process that explored the use of graphene oxide (GO) as a catalyst in the hydrothermal carbonization (HTC) process of low-value, high moisture-containing corn fiber (CF) to analyze the morphology, surface area, and porosity characteristics of activated carbon (AC) derived from GO-assisted hydrochar. The SEM results showed significant alteration to the hydrochar morphology revealing carbon spheres with flakes or platelet-like structures when GO was added to the process, which led to increased carbonization and promoted the hydrochar surface area. The surface areas of the ACs produced from the hydrochars were further increased, and a well-developed porous structure was produced with significant micropore volume. The highest surface area of 2549.1 m 2 /g obtained for the AC derived from the hydrochar with the highest GO ratio. Despite the absence of a strong trend between the GO ratio and AC surface area, the SEM analysis and pore size results revealed that the ACs derived from the GO-assisted hydrochars had more intact structures and smaller micropores with interconnected pore channels which would be very favorable for hydrogen storage capacity. The nitrogen content in the ACs was also found to be comparable or higher than carbons from other studies using nitrogen doping steps and was detected in surface functional groups through FT-IR and XPS analysis. Overall, the developed process provides valuable insight into the influence of GO for tailoring porous carbon materials to enhance surface area and pore structure in low-cost and effective bio-based adsorbents, offering opportunities for emerging applications while promoting circular economy principles.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.065
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.238
Teacher spread0.226 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it