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Record W4399282316 · doi:10.1080/00268976.2024.2356750

Dibridged, monobridged, Y-shaped and linear structures of A <sub>2</sub> H <sub>2</sub> molecules, with A = H, Li, Be, B, C, N, O and F. From acetylene to vinylidene

2024· article· en· W4399282316 on OpenAlexaff
Friedrich Grein

Bibliographic record

VenueMolecular Physics · 2024
Typearticle
Languageen
FieldPhysics and Astronomy
TopicAdvanced Chemical Physics Studies
Canadian institutionsUniversity of New Brunswick
Fundersnot available
KeywordsAcetyleneMoleculeChemistryCrystallographyLinear molecular geometryPhysicsMaterials scienceOrganic chemistry

Abstract

fetched live from OpenAlex

CCSD(T)/aug-cc-pVQZ studies were performed on geometries and properties of dibridged, monobridged, Y-shaped (vinylidene-like) and linear HAAH and AHAH structures of A2H2 molecules, with A = H, Li, Be, B, C, N, O and F. Both singlet and triplet structures were studied for O2H2, only triplet structures for B2H2 and only singlet structures for the other molecules. Stable dibridged structures were obtained for Li2H2, Be2H2 and C2H2, stable monobridged structures for B2H2, C2H2, singlet and triplet O2H2. Be2H2, B2H2, C2H2 and N2H2 have stable Y-shaped structures with A-A as axis (A-AH2), whereas B2H2 and triplet O2H2 also have stable Y-shaped structures with H-H as axis (slightly distorted for O2H2). Stable structures with large interatomic distances were found, such as monobridged singlet and triplet O···HOH in Cs symmetry, Y-shaped Be···BeH2, B···BH2, H···HB2 in C2v symmetry and H···HO2 in Cs symmetry, as well as linear HBe···BeH and Be···HBeH. The energy difference between monobridged C2H2 and vinylidene ­is 1.395 kcal/mol with CCSD(T)/aug-cc-pVQZ and 1.363 kcal/mol with CCSD(T)/aug-cc-pV5Z.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.145
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.222
Teacher spread0.215 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2024
Admission routes1
Has abstractyes

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