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Record W4399369804 · doi:10.1002/adfm.202404995

3D Digital Holography Investigations of Giant Photostriction Effect in MAPbBr<sub>3</sub> Perovskite Single Crystals

2024· article· en· W4399369804 on OpenAlexaff
Dong Liu, Jialin Wu, Ying‐Bo Lu, Yiyang Zhao, Xianyuan Jiang, Kai‐Li Wang, Hao Wang, Liang Dong, Wei‐Yan Cong, Hao Chen, Zhijun Ning, Zhao‐Kui Wang, ChengBo Guan, Zhongchen Wu, Zongcheng Ling

Bibliographic record

VenueAdvanced Functional Materials · 2024
Typearticle
Languageen
FieldEngineering
TopicPerovskite Materials and Applications
Canadian institutionsUniversity of Toronto
FundersNatural Science Foundation of Shandong ProvinceNational Natural Science Foundation of China
KeywordsMaterials sciencePerovskite (structure)HolographyCondensed matter physicsSingle crystalCrystallographyOpticsPhysics

Abstract

fetched live from OpenAlex

Abstract The photoinduced physics always is a critical but controversial question for the new optoelectronic materials of halide perovskites. A high‐quality MAPbBr 3 single crystal is grown and the lattice expansion induced by variable power X‐ray irradiation is investigated.A photoinduced deformation measurement system utilizing the off‐axis holography technique is developed and constructed to measure and illuminate the global photo‐induced deformation of MAPbBr 3 . Under a 473 nm laser with a power of 50 mW, MAPbBr 3 exhibits an average maximum relative deformation of 1.27 × 10 −3 , demonstrating its remarkable photosensitivity and robust geometric response capabilities. Digital holography reveals photostriction as a localized phenomenon, reflecting the localization effect of the photogenerated carriers. The energetic and spatial transitions of those photogenerated carriers weaken the interatomic forces and in turn straighten the Pb─Br─Pb frameworks, expanding the lattice. This geometric change and the corresponding electronic impact are verified by Raman spectra, photoluminescence measurements, and first‐principle calculations. The methods and results are significant for future research on light‐induced phenomena in perovskites and other solid materials.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.007
Threshold uncertainty score0.887

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.190
Teacher spread0.184 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2024
Admission routes1
Has abstractyes

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