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Record W4399479778 · doi:10.1021/acsaom.4c00194

Exploring the Synergistic Properties of ZnGa<sub>2</sub>O<sub>4</sub>:Cr<sup>3+</sup> and Calcium Phosphate: Longer-Lasting Persistent Luminescent Nanocomposite Using Adenosine Triphosphate As a Phosphorus Source

2024· article· en· W4399479778 on OpenAlexafffund
Clement Lee, Yihong Liu, Yasmeen Shamiya, Arghya Paul, Lijia Liu

Bibliographic record

VenueACS Applied Optical Materials · 2024
Typearticle
Languageen
FieldMaterials Science
TopicLuminescence Properties of Advanced Materials
Canadian institutionsWestern University
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsPhosphorusNanocompositeCalciumPhosphateLuminescenceInorganic chemistryChemistryMaterials scienceNuclear chemistryRadiochemistryNanotechnologyMetallurgyBiochemistryOptoelectronics

Abstract

fetched live from OpenAlex

Near-infrared persistent luminescence (PersL) nanoparticles are an emerging type of biomaterial that can continuously emit tissue-penetrable light. Surface functionalization techniques to improve the biological suitability of the phosphor often lead to a noticeable decrease in the luminescence capabilities of the material. In this work, Cr 3+ -doped ZnGa 2 O 4 (CZGO) nanoparticles are incorporated into an amorphous calcium phosphate (ACP) matrix to form a nanocomposite. Utilizing adenosine triphosphate (ATP) as an organic phosphorus source, the luminescence of the CZGO@ACP composite is much brighter and longer-lasting compared to bare CZGO. We found that these improved optical properties were present only when an organic phosphorus source (instead of the conventional inorganic phosphate salt, (NH 4 ) 2 HPO 4 ) was used as the ACP precursor. The chemical structure of the composite synthesized using ATP was comparatively studied with that synthesized using (NH 4 ) 2 HPO 4 . We use X-ray absorption fine structure to unravel the unique interaction between CZGO and ATP. Lastly, in vitro cytocompatibility and antibacterial tests were also performed to assess the biocompatibility of this nanocomposite.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Scholarly communication
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.006
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0020.000
Bibliometrics0.0000.001
Science and technology studies0.0010.001
Scholarly communication0.0020.001
Open science0.0010.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.043
GPT teacher head0.233
Teacher spread0.190 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2024
Admission routes2
Has abstractyes

Explore more

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