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Record W4399873376 · doi:10.1021/acsaelm.4c00509

Nitrogen-Doped Graphene-Ti<sub>3</sub>C<sub>2</sub>T<sub><i>x</i></sub> Quasi-3D Heterostructures Interfacial Interaction for High-Temperature Vibrational Piezoelectric Energy Harvesting Application

2024· article· en· W4399873376 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueACS Applied Electronic Materials · 2024
Typearticle
Languageen
FieldMaterials Science
TopicMXene and MAX Phase Materials
Canadian institutionsUniversity of Calgary
Fundersnot available
KeywordsPiezoelectricityMaterials scienceHeterojunctionDopingNitrogenGrapheneOptoelectronicsNanotechnologyComposite materialChemistry

Abstract

fetched live from OpenAlex

Piezoelectric nanogenerators (PENG) can face challenges when integrated into high-temperature applications because of their high-temperature sensitivity. Heterostructures of specific 2D nanomaterials can potentially enhance the PENG performance for practical applications at high temperatures. Hence, this study incorporates nitrogen-doped graphene (NGr) and Ti 3 C 2 T x MXene heterostructure nanofillers into the polyvinylidene difluoride (PVDF) matrix for energy harvesting in a high-temperature vibration environment. The reproducible and stable all-solution fabrication is achieved by optimizing the appropriate ratio of the NGr-Ti 3 C 2 T x ratio. At room temperature, the nanogenerator showed an optimum output voltage of ∼9.0 V and ∼1.5 μA of current. Thereby, it increased to 24.0 V and 1.75 μA when the temperature increased to 90 °C, obtaining a power density of 3.85 μW/cm 2 . This outstanding performance is attributed to the designed NGr-Ti 3 C 2 T x quasi-3D heterostructure, where its rich interfacial features, excellent electrical conductivity, and localized elastic complexes synergistically promote the piezoelectric output of the energy harvester. Placing the device on the road could be used to collect the mechanical energy generated by the vibration of the car’s movement and convert it into electrical energy, which opens up new development possibilities for addressing emerging energy issues.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Scholarly communication
Consensus categoriesMeta-epidemiology (narrow)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.020
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0010.000
Scholarly communication0.0020.001
Open science0.0010.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.226
Teacher spread0.219 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it