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Record W4400174431 · doi:10.1016/j.csite.2024.104030

Experimental and numerical investigations of soot formation in propane laminar coflow flames in O2/N2 and O2/CO2 atmospheres

2024· article· en· W4400174431 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueCase Studies in Thermal Engineering · 2024
Typearticle
Languageen
FieldChemical Engineering
TopicAdvanced Combustion Engine Technologies
Canadian institutionsnot available
FundersNational Research Council CanadaNational Natural Science Foundation of China
KeywordsSootDiffusion flameCombustionOxygenHydrogenLaminar flowPropaneAcetyleneLimiting oxygen concentrationMaterials scienceAdiabatic flame temperatureChemistryThermodynamicsOrganic chemistryCombustor

Abstract

fetched live from OpenAlex

Oxygen-rich combustion is a new type of clean combustion technology with important application prospects. At present, there are few detailed analyses on the mechanism changes of soot formation under oxygen enrichment of propane. In this paper, the effects of oxygen-rich (O2/N2, O2/CO2) combustion on soot formation in the propane laminar flow coaxial jet diffusion flame were investigated by using the experiment and numerical simulation. The flame image was taken by a color (CCD) camera in the visible band, and the two-dimensional distribution of temperature and soot volume fraction in the flame was reconstructed. In numerical simulation, the soot production model considers a detailed description of nucleation via collisions among heavy polycyclic aromatic hydrocarbons, particle aggregation, polycyclic aromatic hydrocarbons condensation, surface growth and oxidation through the hydrogen abstraction acetylene addition mechanism. The results show that the experimental results were compared with the numerical simulation results, and the numerical simulation results predict the temperature and soot change of oxygen-rich flame well. With the increase in oxygen concentration, the peaks of soot and temperature in the two oxygen-rich atmospheres gradually increased. With the increase in oxygen concentration, the peaks of soot and temperature in the two oxygen-rich atmospheres gradually increased. Comparing the combustion mechanism changes of the two oxygen-rich combustion systems, it was found that the hydrogen abstraction acetylene addition mechanism was the main cause of soot generation. The OH oxidation is dominated near the fuel nozzle side, and O2 oxidation is dominant downstream. With the substitution of CO2 for N2, the chemical effect of CO2 reduces the flame temperature and inhibits the formation mechanism and oxidation mechanism of soot to some extent. This in turn leaded to a reduction in the amount of soot produced.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.068
Threshold uncertainty score0.711

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.020
GPT teacher head0.276
Teacher spread0.256 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it