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Record W4400248251 · doi:10.1038/s44296-024-00016-w

A short review on green H2 production by aqueous phase reforming of biomass derivatives

2024· review· en· W4400248251 on OpenAlexafffund
Songqi Leng, Shahzad Barghi, Chunbao Xu

Bibliographic record

Venuenpj Materials Sustainability · 2024
Typereview
Languageen
FieldChemical Engineering
TopicCatalysts for Methane Reforming
Canadian institutionsWestern University
FundersNatural Sciences and Engineering Research Council of CanadaChina Scholarship Council
KeywordsHydrogen productionCatalysisEnvironmentally friendlySteam reformingBiomass (ecology)Fossil fuelHydrogenMaterials scienceEnvironmental scienceWaste managementChemical engineeringChemistryOrganic chemistryEngineering

Abstract

fetched live from OpenAlex

Abstract Due to high energy content and environmentally friendly attributes, hydrogen is regarded as an ideal energy carrier, serving as a viable alternative to fossil fuels. Steam reforming of fossil fuels is currently the dominant source of hydrogen production with negative environmental impacts, therefore aqueous phase reforming (APR) of biomass derivatives represents an attractive method for green hydrogen production due to its relatively mild operating temperatures and carbon neutrality. This work provides an overview of the types of catalysts employed in the APR process and their pros and cons regarding their performance and operating conditions. Effects of various catalyst supports, e.g., alloy oxides, composite active metals and ceria, and feedstocks, on performance of the catalysts in APR are also discussed. Recent advances and challenges in APR are summarized into several aspects, (1) doping metals/inorganics into support, (2) structural manipulation and defect induction to support, (3) synthesis of single-atom catalysts, (4) development of more eco-friendly processes or catalysts. The present review can provide guidance for prospective development of efficient catalysts and supports for APR of biomass derivatives for green H2 production.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.006
Threshold uncertainty score0.020

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0020.003
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0060.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.032
GPT teacher head0.368
Teacher spread0.336 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations22
Published2024
Admission routes2
Has abstractyes

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