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Record W4400594945 · doi:10.1002/cjce.25392

A simultaneous study on desulphurization and denitrogenation using acid‐treated activated alumina: Multi‐component adsorption systems

2024· article· en· W4400594945 on OpenAlexvenueno aff
Naushad Khan, G.Karthik Reddy, Sandeep Kumar Thaligari, Vimal Chandra Srivastava, Raj Singh, Anuj Rawat, Paritosh Mohanty

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2024
Typearticle
Languageen
FieldEngineering
TopicCatalysis and Hydrodesulfurization Studies
Canadian institutionsnot available
Fundersnot available
KeywordsAdsorptionComponent (thermodynamics)ChemistryFlue-gas desulfurizationChemical engineeringChromatographyOrganic chemistryThermodynamicsEngineering

Abstract

fetched live from OpenAlex

Abstract In this study, sulphuric acid‐treated activated alumina (AA) was used for sulphur and nitrogen removal from model fuel in a batch adsorption study. Dibenzothiophene (DBT), a sulphur compound, and quinoline, a nitrogen compound dissolved in isooctane, were taken as a model liquid fuel. Detailed characterization of the adsorbent, such as scanning electron microscopy (SEM), thermogravimetric analysis‐differential thermal analysis (TGA‐DTA), Fourier transform infrared spectroscopy (FTIR), Brunauer–Emmett–Teller (BET), and X‐ray diffraction (XRD), was performed to understand the DBT and quinoline adsorption mechanism onto AA adsorbent. Sulphur and nitrogen removal efficiencies were found to be 64% and 91%, respectively. Mono‐component adsorption isotherm was studied by using different models such as Langmuir, Freundlich, and Redlich‐Peterson (R‐P) isotherms. The R‐P isotherm model well‐predicted the individual equilibrium data for both nitrogen and sulphur from the liquid fuel. Binary‐component adsorption studies were performed by mixing both DBT and quinoline in isooctane. Binary‐equilibrium data were modelled by multi‐component models such as modified Langmuir isotherm, non‐modified Langmuir, extended Langmuir, extended Freundlich isotherm, Sheindorf‐Rebuhn‐Sheintuch (SRS), non‐modified R‐P model, and modified R‐P model. The extended Freundlich (E‐F) adsorption isotherm model was found to best fit the binary equilibrium system.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.217
Teacher spread0.201 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2024
Admission routes1
Has abstractyes

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