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Record W4401027280 · doi:10.1002/smll.202402464

Enhanced Sensitivity in Photovoltaic 2D MoS <sub>2</sub> /Te Heterojunction VOC Sensors

2024· article· en· W4401027280 on OpenAlexafffund
Mohammad Reza Mohammadzadeh, Amirhossein Hasani, Tanveer Hussain, Hamidreza Ghanbari, Mirette Fawzy, Amin Abnavi, Ribwar Ahmadi, Fahmid Kabir, Thushani De Silva, R. K. N. D. Rajapakse, Michael M. Adachi

Bibliographic record

VenueSmall · 2024
Typearticle
Languageen
FieldEngineering
TopicGas Sensing Nanomaterials and Sensors
Canadian institutionsSimon Fraser University
FundersWestern Economic Diversification CanadaBritish Columbia Knowledge Development FundCMC MicrosystemsWorkSafeBCNatural Sciences and Engineering Research Council of CanadaCanada Foundation for Innovation
KeywordsHeterojunctionMaterials scienceSensitivity (control systems)OptoelectronicsPhotovoltaic systemFlexibility (engineering)NanotechnologyElectronic engineeringElectrical engineering

Abstract

fetched live from OpenAlex

Abstract Volatile organic compound (VOC) sensors have a broad range of applications including healthcare monitoring, product quality control, and air quality management. However, many such applications are demanding, requiring sensors with high sensitivity and selectivity. 2D materials are extensively used in many VOC sensing devices due to their large surface‐to‐volume ratio and fascinating electronic properties. These properties, along with their exceptional flexibility, low power consumption, room‐temperature operation, chemical functionalization potential, and defect engineering capabilities, make 2D materials ideal for high‐performance VOC sensing. Here, a 2D MoS 2 /Te heterojunction is reported that significantly improves the VOC detection compared to MoS 2 and Te sensors on their own. Density functional theory (DFT) analysis shows that the MoS 2 /Te heterojunction significantly enhances the adsorption energy and therefore sensing sensitivity of the sensor. The sensor response, which denotes the percentage change in the sensor's conductance upon VOC exposure, is further enhanced under photo‐illumination and zero‐bias conditions to values up to ≈7000% when exposed to butanone. The MoS 2 /Te heterojunction is therefore a promising device architecture for portable and wearable sensing applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.080
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.189
Teacher spread0.179 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations18
Published2024
Admission routes2
Has abstractyes

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