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Record W4401047833 · doi:10.1016/j.epsl.2024.118899

Ultramafic melt viscosity: A model

2024· article· en· W4401047833 on OpenAlexafffund
James K. Russell, Kai‐Uwe Hess, Donald B. Dingwell

Bibliographic record

VenueEarth and Planetary Science Letters · 2024
Typearticle
Languageen
FieldMaterials Science
TopicMaterial Dynamics and Properties
Canadian institutionsUniversity of British Columbia
FundersH2020 European Research CouncilEuropean Research CouncilNatural Sciences and Engineering Research Council of CanadaAlexander von Humboldt-Stiftung
KeywordsGeologyUltramafic rockViscosityGeophysicsGeochemistryPetrologyThermodynamics

Abstract

fetched live from OpenAlex

A non-Arrhenian model for the Newtonian viscosity (η) of ultramafic melts is presented. The model predicts the viscosity of ultramafic melts as a function of temperature (T), pressure (P), H2O content and for a range of melt compositions (70 < Mg# < 100). The calibration consists of 63 viscosity measurements at ambient pressure for 20 individual melt compositions and 5 high-P measurements on a single melt composition, all drawn from the literature. The data span 14 orders of magnitude of η (10−2 to 1011.8 Pa s), a T range of 880 to 2700 K, pressures from 1 atm to 25 GPa, and include measurements on hydrous melts containing 0.2 to 4.4 wt.% H2O. The T-dependence of viscosity is modelled with the VFT equation [log η = A + B/(T(K) − C)] whereby A is assumed to be a common, high-T limit for these melt compositions (i.e. log η∞ = -5.4). The pressure and composition effects are parameterised in terms of 5 adjustable parameters in expanded forms of B and C. The viscosity model is continuous across T-P-composition space and can predict ancillary transport properties including glass transition temperatures (Tg) and melt fragility (m). Melt viscosity decreases markedly with increasing H2O content but increases significantly with increasing pressure and decreasing Mg# (i.e. higher Fe-content). We show strong systematic decreases in Tg and m with increasing H2O content whereas an increase in P causes a rise in Tg and decrease in m. The predictive capacity of this model for ultramafic melt viscosity makes it pertinent to the fields of volcanology, geophysics, petrology, and the material sciences. Moreover, it provides constraints on models of magma oceans on terrestrial planets and, the evolution of planetary atmospheres via magmatic degassing on exoplanets.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.906
Threshold uncertainty score0.706

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.191
Teacher spread0.182 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2024
Admission routes2
Has abstractyes

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