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Record W4401338585 · doi:10.1103/physrevb.110.064405

Field-induced transformation of complex spin ordering and magnetodielectric and magnetoelastic coupling in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>MnGeTeO</mml:mi><mml:mn>6</mml:mn></mml:msub></mml:mrow></mml:math>

2024· article· lv· W4401338585 on OpenAlexfundno aff
Y. H. Chang, Arkadeb Pal, Peter Tsung-Wen Yen, Chin‐Wei Wang, Sanjib Giri, Graeme R. Blake, Javier Gainza, M.-J. Hsieh, J. Y. Lin, Chin‐Yu Huang, Yi–Ju Chen, T. W. Kuo, Ajay Tiwari, D. Chandrasekhar Kakarla, H. D. Yang

Bibliographic record

VenuePhysical review. B./Physical review. B · 2024
Typearticle
Languagelv
FieldMaterials Science
TopicMultiferroics and related materials
Canadian institutionsnot available
FundersScience and Engineering Research BoardEnvironmental Studies Research FundsHORIZON EUROPE Marie Sklodowska-Curie ActionsNational Science and Technology Council
KeywordsCoupling (piping)Field (mathematics)Transformation (genetics)Spin (aerodynamics)Condensed matter physicsPhysicsMaterials scienceMathematicsChemistryPure mathematicsThermodynamics

Abstract

fetched live from OpenAlex

Spin-frustrated systems are well known for exhibiting fascinating and exotic magnetic properties and are often intertwined with other intriguing phenomena. Magnetization and specific-heat studies suggest that the spin-frustrated chiral triangular lattice compound ${\mathrm{MnGeTeO}}_{6}$ undergoes a long-range antiferromagnetic transition below the N\'eel temperature $({T}_{\mathrm{N}})$ \ensuremath{\sim} 9 K, which is further validated in the neutron powder-diffraction (NPD) study. In the absence of an external magnetic field $(H)$, analysis of NPD data reveals a complex incommensurate spin structure, characterized by a mixture of helical and cycloidal spin orderings with a propagation vector of $\mathbit{k}=(1/3, 1/3, 0.184)$. Upon the application of $H$, this spin ordering transforms into a conical spin structure, which is manifested as a metamagnetic transition in the isothermal magnetization $(M)$ curve when $H$ exceeds \ensuremath{\sim} 0.9 T. Total energy calculations and estimation of various exchange-interaction energies $(J)$ by density-functional theory calculations also support the formation of such a complex spin ordering. Moreover, a pronounced dielectric $({\ensuremath{\varepsilon}}^{\ensuremath{'}})$ anomaly is observed near ${T}_{\mathrm{N}}$, which is suppressed considerably under H. The variation of ${\ensuremath{\varepsilon}}^{\ensuremath{'}}$ with increasing H closely reflects the $\mathrm{\ensuremath{\Delta}}{\ensuremath{\varepsilon}}^{\ensuremath{'}}\phantom{\rule{4pt}{0ex}}\ensuremath{\propto}$ ${M}^{2}$ scaling behavior in the low-H regime, thus indicating a higher-order magnetoelectric coupling. Moreover, synchrotron x-ray diffraction reveals an isostructural distortion below ${T}_{\mathrm{N}}$, suggesting magnetoelastic coupling as a trigger for the dielectric anomaly.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.799
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0160.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.025
GPT teacher head0.298
Teacher spread0.273 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2024
Admission routes1
Has abstractyes

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