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Record W4401609898 · doi:10.1016/j.chemer.2024.126174

Microstructural control on the trace element distribution and Au concentration in pyrite nodules

2024· article· en· W4401609898 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.
aboutThe title or abstract carries a Canadian signal from the geographic lexicon.

Bibliographic record

VenueGeochemistry · 2024
Typearticle
Languageen
FieldComputer Science
TopicGeochemistry and Geologic Mapping
Canadian institutionsGeological Survey of CanadaNatural Resources Canada
FundersNatural Resources CanadaFirst Quantum Minerals
KeywordsPyriteTrace elementMineralogyGeologyHematiteGrain boundaryMicrostructureGeochemistryMaterials scienceMetallurgy

Abstract

fetched live from OpenAlex

The crystal growth history of an Au-rich sedimentary pyrite nodule from the Timmins-Porcupine Au camp, Ontario, Canada, has been investigated using Electron Backscattered Diffraction and Laser Ablation Inductively Coupled Plasma Mass Spectrometry techniques to study the crystallographic processes controlling metal deportment in the pyrite structure. Results show four distinct growth stages characterized by different pyrite microstructures, crystal forms and trace element compositions. A direct link is observed between the growth of octahedral facets in pyrite and the development of primary (non-tectonic) subgrain boundaries. Furthermore, zones with a high abundance of subgrain boundaries have the highest Au, As, Ag and Cu (and other metals) contents – suggesting metal distribution is linked to the development of microstructures. Finer-grained aggregates are characterized by higher grain boundary density than in coarse areas, making higher trace element concentrations inversely proportional to grain size. Our results indicate that the high Au concentrations (~100 ppm) in pyrite represent a primary feature related to nodule growth, instead of secondary enrichment processes, and highlight the possibility that sediment-hosted pyrite nodules could represent a metal-rich geochemical reservoir for the formation of younger orogenic Au deposits. • Microstructures in diagenetic pyrite nodules are linked to metal incorporation. • Au, As, Ag, and Cu are concentrated in non-tectonic grain and subgrain boundaries. • Grain and subgrain boundaries are interpreted as primary growth structures. • The incorporation of Au, As, Ag, is a primary feature in diagenetic pyrite nodules. • High S content during diagenesis is related with higher Au incorporation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.176
Threshold uncertainty score0.353

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.209
Teacher spread0.202 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it