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Record W4401834352 · doi:10.3390/ma17164126

Conductive Polymer-Based Electrodes and Supercapacitors: Materials, Electrolytes, and Characterizations

2024· review· en· W4401834352 on OpenAlexafffund
Zahra Roohi, Frej Mighri, Ze Zhang

Bibliographic record

VenueMaterials · 2024
Typereview
Languageen
FieldMaterials Science
TopicSupercapacitor Materials and Fabrication
Canadian institutionsUniversité LavalHôpital Saint-François d'Assise
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsSupercapacitorMaterials scienceConductive polymerPolyanilinePolypyrroleCarbon nanotubeCyclic voltammetryElectrolytePolythiopheneEnergy storageNanotechnologyPseudocapacitorGrapheneDielectric spectroscopyPolymerElectrochemistryElectrodeComposite materialChemistry

Abstract

fetched live from OpenAlex

New materials and the interactions between them are the basis of novel energy storage devices such as supercapacitors and batteries. In recent years, because of the increasing demand for electricity as an energy source, the development of new energy storage materials is among the most actively studied topics. Conductive polymers (CPs), because of their intrinsic electrochemical activity and electrical conductivity, have also been intensively explored. While most of the high capacitance reported in the literature comes from hybrid materials, for example, conductive polymers composed of metal oxides and carbon materials, such as graphene and carbon nanotubes, new chemistry and the 3D structure of conductive polymers remain critical. This comprehensive review focuses on the basic properties of three popular conductive polymers and their composites with carbon materials and metal oxides that have been actively explored as energy storage materials, i.e., polypyrrole (PPy), polyaniline (PANi), and polythiophene (PTh), and various types of electrolytes, including aqueous, organic, quasi-solid, and self-healing electrolytes. Important experimental parameters affecting material property and morphology are also discussed. Electrochemical and analytical techniques frequently employed in material and supercapacitor research are presented. In particular, cyclic voltammetry (CV) and electrochemical impedance spectroscopy (EIS) are discussed in detail, including how to extract data from spectra to calculate key parameters. Pros and cons of CP-based supercapacitors are discussed together with their potential applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Scholarly communication, Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.173
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0030.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0020.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0020.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.033
GPT teacher head0.288
Teacher spread0.255 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations38
Published2024
Admission routes2
Has abstractyes

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