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Record W4401883944 · doi:10.1021/acsaelm.4c00859

Green-Solvent-Based Conductive Graphene Ink Prepared via Liquid-Phase Exfoliation of Graphite with Water-Soluble 2,6-Azulene-Based Copolymers as Stabilizers

2024· article· en· W4401883944 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueACS Applied Electronic Materials · 2024
Typearticle
Languageen
FieldMaterials Science
TopicGraphene research and applications
Canadian institutionsUniversité Laval
FundersNatural Sciences and Engineering Research Council of CanadaCentre québécois sur les matériaux fonctionnels
KeywordsMaterials scienceCopolymerGrapheneExfoliation jointChemical engineeringConductive inkRaman spectroscopyAzuleneGraphiteSolventNanotechnologyComposite materialSheet resistancePolymerOrganic chemistryChemistry

Abstract

fetched live from OpenAlex

Liquid-phase exfoliation (LPE) of graphite is a promising strategy to prepare stabilized graphene inks for various applications. However, the stabilizing agents that have been used generally suffer from poor electrical properties, harming the properties of the resulting composites once they are deposited on a surface. In this study, we investigate the use of a water-soluble, conjugated 2,6-azulene-based copolymer as a stabilizing agent for aqueous graphene dispersion. Due to the presence of azulene within the copolymer main chain, the copolymer exhibits proton responsiveness and conductivity in the solid state upon protonation. The LPE process was optimized in a mixture of water and ethanol (1:1), and stable inks can be obtained after 2 h of sonication using a copolymer concentration as low as 0.09 mg·mL –1 . The resulting inks were deposited on various surfaces and characterized using Raman spectroscopy, UV–visible spectroscopy, and atomic force microscopy (AFM), which led us to conclude that few- and multilayer graphenes were obtained. Finally, the optimized ink was printed on glossy photographic paper using a modified FDM 3D printer to create printed circuits with a sheet resistance of 60 kΩ·□ –1 .

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.011
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.276
Teacher spread0.266 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it