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Record W4401908320 · doi:10.1021/acsestair.4c00128

Spatiotemporally Detailed Quantification of Air Quality Benefits of Emissions–Part II: Sensitivity to Study Parameters and Assumptions

2024· article· en· W4401908320 on OpenAlexaff
Amir Hakami, Shunliu Zhao, Petros Vasilakos, Anas Alhusban, Yaşar Burak Öztaner, Alan Krupnick, Howard H. Chang, Armistead G. Russell

Bibliographic record

VenueACS ES&T Air · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicAir Quality and Health Impacts
Canadian institutionsCarleton University
FundersHealth Effects InstituteNational Aeronautics and Space Administration
KeywordsCMAQEnvironmental scienceAir quality indexParticulatesNOxAtmospheric sciencesPopulationMeteorologyClimatologyEnvironmental healthGeographyChemistryGeologyMedicine

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide Adjoint modeling, using U.S. EPA’s Community Multiscale Air Quality (CMAQ), has been performed to provide location-specific monetized health benefits from the controls of primary PM 2.5 and PM 2.5 precursors (NO x, SO 2, and NH 3 ) across North America. Source-to-health benefit relationships are quantified using a benefit-per-ton (BPT) metric, accounting for the impacts on premature mortality due to long-term exposure to fine particulate matter. In the base analysis, the approach used a 12 km resolution, four 2-week episodes chosen to capture annual responses, emissions for 2016, and the Global Exposure Mortality Model (GEMM) to link exposures to premature mortality. Here, we investigate the impacts those choices have on results using a range of sensitivity analyses. The choice of four representative episodes led to relatively little bias and error. Finer model resolution, investigated by comparing 36, 12, 4, and 1 km simulations over two urban areas, tended to increase BPT estimates, though the impact was inconsistent between different regions. While BPTs and burden estimates were consistent across resolutions over New York City, they sharply increased for Los Angeles, particularly for NOx and ammonia, leading to 90% increase in burden estimates at 1 km resolution. We find that, for primary PM 2.5 emissions, better resolved population distribution is the main contributing factor to higher BPTs, but for secondary precursor emissions (ammonia and NOx), higher model resolution that avoids dilution in coarser grids is more important. Changing emissions from 2016 to 2001 and 2028 resulted in fairly consistent primary PM 2.5 BPTs but impacted the BPTs for NOx and ammonia more significantly due to changes in SO 2 emissions. We found that BPTs tend to stabilize, as emission changes in 2028 lead to a lower deviation from 2016 BPTs compared to changes from the 2001 episode. The role of the epidemiological model also led to relatively modest uncertainties, 15–30% depending on the species, even when different shapes of concentration–response functions were employed. We found the impact of the choice of CRF to be larger or comparable in size to the reported epidemiological model uncertainties for log–linear CRFs. The adjoining approach proved robust to modeling choices in providing BPT estimates that are highly granular across locations and emitted species.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.191
Threshold uncertainty score0.461

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.098
GPT teacher head0.362
Teacher spread0.264 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2024
Admission routes1
Has abstractyes

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