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Record W4402176912 · doi:10.1088/2053-1591/ad76fe

Ultrasonic assisted removal of methyl orange and bovine serum albumin from wastewater using modified activated carbons: RSM optimization and reusability

2024· article· en· W4402176912 on OpenAlexaff
Imran Ahmad Khan, Asad Ullah Khan, Kashif Mairaj Deen, Edouard Asselin, Rehan Sadiq, Muhammad Yasir, Nasir M. Ahmad

Bibliographic record

VenueMaterials Research Express · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicAdsorption and biosorption for pollutant removal
Canadian institutionsUniversity of British Columbia, Okanagan CampusUniversity of British Columbia
FundersHigher Education Commision, PakistanNational University of Sciences and TechnologyHigher Education Commission, Pakistan
KeywordsAdsorptionResponse surface methodologyCentral composite designActivated carbonChemistryBovine serum albuminLangmuir adsorption modelWastewaterMethyl orangeSonicationNuclear chemistryChromatographyChemisorptionOrganic chemistryEnvironmental engineeringPhotocatalysisCatalysis

Abstract

fetched live from OpenAlex

Abstract The removal of industrial pollutants from water remains a significant challenge in water treatment processes. This study investigated the efficacy of powder-activated carbon (PAC), thermally modified PAC (TPAC), and chemically modified PAC (CPAC) for removing bovine serum albumin (BSA) and methyl orange (MO) from simulated wastewater. After undergoing treatment, the BET surface area of TPAC increased to 823 m 2 g −1 , while that of CPAC increased to 657 m 2 g −1 compared to the initial surface area of pristine PAC, which was 619 m 2 g −1 . Batch adsorption experiments assisted by ultrasonication were conducted to evaluate the impact of solution pH, initial concentration, and contact time on the adsorption capacities ( q max ) of BSA and MO. TPAC demonstrated superior performance, achieving q max values of 152 mg g −1 for MO and 133 mg g −1 for BSA, compared to PAC, which provided q max values of 124 mg g −1 and 112 mg g −1 , respectively. Furthermore, pH levels of 3 and 5 were identified as highly effective for the removal of MO and BSA from water, respectively. The adsorption kinetics of both MO and BSA followed pseudo2nd-order ( R 2 > 0.99) reaction kinetics under both batch and ultrasonic conditions, confirming the removal of contaminants through chemisorption. The adsorption trends also satisfied the Langmuir isothermal model, indicating the formation of a uniform monolayer during the adsorption process of these contaminants. To understand the simultaneous effect of all the variables, response surface methodology (RSM) using central composite design (CCD) was used to predict the adsorption capacities of CPAC. After five adsorption cycles, the removal efficiencies of MO (from 98% to 80%) and BSA (from 55% to 40%) decreased in the CPAC system. The results suggested that CPAC can be effectively utilized to remove MO from wastewater.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.016
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.063
GPT teacher head0.325
Teacher spread0.262 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2024
Admission routes1
Has abstractyes

Explore more

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