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Record W4402509929 · doi:10.1016/j.cej.2024.155714

The role of nanodimensions in enhancing electrochemical sensing: A comprehensive review

2024· review· en· W4402509929 on OpenAlexafffund
Melika Jalali, Seyed Morteza Hosseini‐Hosseinabad, Roozbeh Siavash Moakhar, Mahsa Jalali, Mohammad Mirzaei, Sunny Kumar Sharma, Alireza Sanati, Sahar Sadat Mahshid, Yogendra Kumar Mishra, Sara Mahshid

Bibliographic record

VenueChemical Engineering Journal · 2024
Typereview
Languageen
FieldEngineering
TopicElectrochemical sensors and biosensors
Canadian institutionsMcGill University
FundersDanish Agency for Science and Higher EducationNatural Sciences and Engineering Research Council of CanadaFonds de recherche du QuébecMcGill UniversityCanada Excellence Research Chairs, Government of CanadaCanada Foundation for InnovationCanada Research Chairs
KeywordsElectrochemistryEnvironmental scienceMaterials scienceNanotechnologyChemistryElectrode

Abstract

fetched live from OpenAlex

Catalytic sensing of molecular biomarkers has become increasingly important in health monitoring and point-of-care diagnostics due to their promising properties. To develop technology for catalytic sensing of molecular biomarkers, financial and environmental sustainability must be considered. Small-molecule biomarkers play a crucial role in numerous physiological processes and are commonly utilized for disease detection by monitoring cell signaling, bioprocesses, cell viability, metabolomics, and pharmacokinetics. Nanostructured materials with varied dimensions have been extensively utilized in molecular sensing, capitalizing on their enhanced electrocatalytic activities. As a result of significant advancements in materials and fabrication technologies, novel nanostructured platforms have been developed in various shapes to accommodate various analytes of interest. The nanostructured platforms can be divided into four main categories based on their dimensionality, including nanoparticles or zero-dimensional (0D), one-dimensional (1D), two-dimensional (2D), and three-dimensional (3D) nanomaterials. Each category of nanomaterials has demonstrated numerous advantages for electrocatalytic sensing due to their extraordinary surface-to-volume ratio and fast electron-hole transfer routes. Still, the existing disadvantages, such as their volatility to chemicals and wetness, hinder their widespread applications in sensing. Despite their advantages, challenges such as susceptibility to chemicals and wetness hinder their widespread use in sensing applications. Recently, the integration of multiscale nanocompositions, particularly 2D functional materials, has drawn attention for enhancing electrocatalytic activity. Our innovative outlook in this review involves integrating multiscale nano compositions, particularly 2D functional materials and fractal nanostructures, to enhance catalytic and electrocatalytic activities. These advancements will drive significant progress in the field of biosensing, offering new solutions for complex diagnostic challenges.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Research integrity
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.853
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0020.001
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.003
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.241
Teacher spread0.233 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designNot applicable
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations27
Published2024
Admission routes2
Has abstractyes

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