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Record W4402589662 · doi:10.1149/1945-7111/ad7c85

Multiphysics Simulation of Multi-layered Fibrous Electrodes for the Vanadium Redox Flow Battery

2024· article· en· W4402589662 on OpenAlexfundno aff
Kyu Min Lee, Mehrzad Alizadeh, Takahiro Suzuki, Shohji Tsushima, Edward P.L. Roberts, Jeff T. Gostick

Bibliographic record

VenueJournal of The Electrochemical Society · 2024
Typearticle
Languageen
FieldEngineering
TopicAdvanced battery technologies research
Canadian institutionsnot available
FundersJapan Society for the Promotion of ScienceNatural Sciences and Engineering Research Council of Canada
KeywordsMultiphysicsVanadiumFlow batteryRedoxElectrodeMaterials scienceBattery (electricity)NanotechnologyChemical engineeringChemistryMetallurgyFinite element methodEngineeringThermodynamicsPhysics

Abstract

fetched live from OpenAlex

Electrospinning can create customized flow-through electrodes for redox flow batteries with small fibers to enhance reactive surface area. A downside is higher pressure drop and parasitic pumping losses. Multilayered electrodes are a promising remedy, but it is not obvious what properties each layer should have to get the most benefit. In this work, a multiphysics simulation was used to explore the impact of varying the properties of each layer on the performance of a cell, including fiber size, fiber alignment, and porosity. The results showed that a 300% increase in limiting current can be obtained over commercial materials when the layer near the membrane has larger fibers with smaller fibers in each successive layer (1.8, 1.0 & 0.2 um, respectively). This arrangement had relatively lower overall efficiency once pumping power was taken into account. A compromise was obtained by placing a high porosity layer near the membrane with lower porosity in each successive layer (91%, 86%, and 81%, respectively). This case resulted in a 250% increase in limiting current, while expending only 0.1% of the output power on pumping.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.921
Threshold uncertainty score0.346

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.279
Teacher spread0.264 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2024
Admission routes1
Has abstractyes

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