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Record W4402770311 · doi:10.1038/s41567-024-02629-3

Electronic response of a Mott insulator at a current-induced insulator-to-metal transition

2024· article· en· W4402770311 on OpenAlexafffund
C. T. Suen, Igor Marković, Marta Zonno, N. Heinsdorf, Sergey Zhdanovich, Na Hyun Jo, M. Schmid, P. Hansmann, Pascal Puphal, K. Fürsich, Steef Smit, C. Au-Yeung, V. Zimmermann, Berend Zwartsenberg, M. Krautloher, Ilya Elfimov, Robert J. Koch, Sergey Gorovikov, Chris Jozwiak, Aaron Bostwick, Marcel Franz, Eli Rotenberg, B. Keimer, A. Damascelli

Bibliographic record

VenueNature Physics · 2024
Typearticle
Languageen
FieldPhysics and Astronomy
TopicAdvanced Condensed Matter Physics
Canadian institutionsCanadian Light Source (Canada)University of British Columbia
FundersLawrence Berkeley National LaboratoryCanadian Institutes of Health ResearchOffice of ScienceUniversity of TokyoMitacsMax-Planck-GesellschaftNatural Sciences and Engineering Research Council of CanadaCanadian Light SourceCanada First Research Excellence FundCanada Research ChairsCanadian Institute for Advanced ResearchNederlandse Organisatie voor Wetenschappelijk OnderzoekBritish Columbia Knowledge Development FundAlexander von Humboldt-StiftungMinistère de la Défense NationaleKillam TrustsU.S. Department of Energy
KeywordsMott insulatorCondensed matter physicsMott transitionMetal–insulator transitionAngle-resolved photoemission spectroscopyPhysicsInsulator (electricity)Photoemission spectroscopyElectronic structurePhase transitionStrongly correlated materialX-ray photoelectron spectroscopyElectronOptoelectronicsElectrical resistivity and conductivityHubbard modelNuclear magnetic resonanceSuperconductivityQuantum mechanics

Abstract

fetched live from OpenAlex

Abstract The Mott insulator Ca 2 RuO 4 exhibits an insulator-to-metal transition induced by d.c. current. Despite the thorough examination of the structural changes associated with this transition, a comprehensive knowledge of the response of electronic degrees of freedom is still lacking. Here we demonstrate current-induced modifications of the electronic states of Ca 2 RuO 4 . Angle-resolved photoemission spectroscopy in conjunction with four-probe electrical transport (transport-ARPES) measurements reveal a clear reduction of the Mott gap and a modification in the dispersion of the Ru bands. Based on a free-energy analysis, we show that the current-induced phase is electronically distinct from the high-temperature zero-current metallic phase. Our results highlight strong interplay of lattice- and orbital-dependent electronic responses in the current-driven insulator-to-metal transition.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.084
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.278
Teacher spread0.272 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2024
Admission routes2
Has abstractyes

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