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Record W4402996719 · doi:10.1021/acs.inorgchem.4c01658

High-Yield Synthesis Route, Post-Synthesis Treatment, and Insights into the Photoluminescence and Magnetic Properties of Tricopper(I) Melaminate Cu<sub>3</sub>(C<sub>3</sub>N<sub>6</sub>H<sub>3</sub>)

2024· article· en· W4402996719 on OpenAlexafffund
Elaheh Bayat, Markus Ströbele, Mojtaba Abbasi, Scott Kroeker, J. Valenta, David Enseling, Thomas Jüstel, Hans‐Jürgen Meyer

Bibliographic record

VenueInorganic Chemistry · 2024
Typearticle
Languageen
FieldChemistry
TopicMetal-Organic Frameworks: Synthesis and Applications
Canadian institutionsUniversity of Manitoba
FundersNatural Sciences and Engineering Research Council of CanadaDeutsche ForschungsgemeinschaftCanada Foundation for Innovation
KeywordsChemistryPhotoluminescenceYield (engineering)CrystallographyStereochemistryOptoelectronicsMetallurgy

Abstract

fetched live from OpenAlex

A novel and more efficient synthesis of Cu 3 (C 3 N 6 H 3 ) is presented through a salt-metathesis reaction using copper(I) chloride and sodium hydrogen cyanamide. This synthesis yields a melaminate trianion through the cyclotrimerization of (HNCN) − ions, offering an alternative route to the deprotonation of melamine for synthesizing melaminate. The reaction is analyzed via differential thermal analysis. After the unconventional formation of this MOF-like structure by solid-state reaction, this material still requires treatment via solvent exchange and vacuum drying due to the presence of a host molecule inside the channels of the structure. The process and the impact of the treatment of Cu 3 (C 3 N 6 H 3 ) on its XRD pattern are thoroughly discussed. Additionally, results from stability, NMR and infrared spectroscopy, and thermogravimetric analysis. Finally, photoluminescence and magnetic studies are conducted to evaluate their potential as a functional material.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.193
Teacher spread0.183 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2024
Admission routes2
Has abstractyes

Explore more

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