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Record W4403097733 · doi:10.1016/j.jece.2024.114353

Behavioral and toxicological impacts of bio-derived oils in aqueous spills

2024· article· en· W4403097733 on OpenAlexaff
Qin Xin, Hena Farooqi, Bassam Al-Haj, Nayereh Saborimanesh

Bibliographic record

VenueJournal of environmental chemical engineering · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicToxic Organic Pollutants Impact
Canadian institutionsNatural Resources Canada
Fundersnot available
KeywordsOil spillEnvironmental chemistryEnvironmental scienceAqueous solutionChemistryWaste managementToxicologyOrganic chemistryEnvironmental engineeringBiologyEngineering

Abstract

fetched live from OpenAlex

There is an increasing global demand for, and transportation of, goods classified as Hazardous and Noxious Substances (HNS), including bio-derived oils and chemicals. With the increasing variety of bio-feedstocks and the development of processing technologies, the physical and chemical properties of commercially available and transported bio-derived oils vary significantly. The objective of this work was to analyze and compare the physical and chemical characteristics, behaviour, and risks of several bio-derived oils (four vegetable oils, one biodiesel, and two pyrolysis oils) and one petrol diesel when spilled into both fresh and salt water system. The laboratory results indicated that the vegetable oils and biodiesel remained buoyant and resulted in low total organic carbon (TOC) in water when spilled, similar behaviour to petrol diesel. However, the two pyrolysis oils exhibited remarkably different behaviours. The two oils sunk directly in the water and then rapidly dissolved the organic components into the water when mixed. This resulted in a high TOC (100 times higher than other types of oil) and an altered water chemistry, leaving a large portion of water-insoluble portion (35.0 wt% of pyrolysis oils) remaining at the water bottom. Initial Microtox findings indicated that water samples contaminated with pyrolysis oils and biodiesel (similar to petrol diesel) exhibited increased aqueous toxicity towards Vibrio fischeri . Further biological tests are required to understand their ecological risks. This work provides insights to the challenges and knowledge gaps on the fate, behaviour and risk of emerging bio-derived oils in water, while supporting HNS emergency response and remediation measures. • Comparison of physical and chemical properties of bio-derived oils to petrol diesel. • Pyrolysis oils exhibit distinct behaviour and will sink and dissolve in water. • Spills of pyrolysis oils result in the highest dissolved organic carbon in water. • Biodiesel and pyrolysis oils have a similar risk to Vibrio fischeri in water.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.081
Threshold uncertainty score0.866

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.217
Teacher spread0.211 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2024
Admission routes1
Has abstractyes

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