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Record W4403141858 · doi:10.26434/chemrxiv-2024-hgwv3

Automated Microcontact Bioprinting for High-Throughput Manufacturing of Lubricant-Infused Microarrays

2024· preprint· en· W4403141858 on OpenAlexafffund
Lubna Najm, Amid Shakeri, Liane Ladouceur, Samantha Dacalos, Sakina Hussain, Inaam Chattha, Hareet Sidhu, Tohid F. Didar

Bibliographic record

VenueChemRxiv · 2024
Typepreprint
Languageen
FieldEngineering
TopicNanofabrication and Lithography Techniques
Canadian institutionsUniversity of TorontoMcMaster University
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsMicrocontact printingLubricantThroughputNanotechnologyMaterials scienceComputer scienceComposite materialOperating system

Abstract

fetched live from OpenAlex

Microarrays are widely used for detecting target analytes and biomarkers, with fabrication methods ranging from non-contact to contact bioprinting techniques. Microcontact bioprinting (μCP), which utilizes elastomeric stamps to transfer biorecognition molecules (bioinks) onto substrates, offers advantages such as customizability, cost-effectiveness, and versatility in handling bioinks with high viscosities. Despite its prevalent use in laboratory settings, μCP faces challenges in achieving the repeatability and reproducibility required for industrial manufacturing. In this study, we address these limitations by developing and optimizing a μCP protocol using industrial techniques. A key innovation in our approach is the combination of microcontact printing with fluorosilanization, enabling the use of lubricant-infused surfaces to prevent non-specific attachment. Additionally, we enhance biomolecule immobilization through covalent attachment using a modified bioink formulation. We identify and mitigate high-risk failure modes including bioink formulation, application and removal, environmental conditions, and force application during stamping. Furthermore, we integrate an automated syringe pump and a standardized force application system, taking critical steps toward industrial scalability. Using lubricant-infused substrates, our optimized μCP protocol demonstrates significant improvements in repeatability and reproducibility, achieving intra-assay and inter-assay coefficients of variance below 10% and signal-to-noise ratios exceeding 15. These advancements validate our μCP method for high-throughput, scalable microarray fabrication, paving the way for its implementation in industrial manufacturing.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.002
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Methods · Consensus signal: Methods
Teacher disagreement score0.001
Threshold uncertainty score0.006

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.002
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0000.001
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.244
Teacher spread0.233 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes2
Has abstractyes

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