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Ice-nucleating particles are emitted by raindrop impact

2024· preprint· en· W4403145115 on OpenAlexfundno aff
Claudia Mignani, Thomas C. J. Hill, Marina Nieto‐Caballero, Kevin R. Barry, Noelle C. Bryan, Peter J. Marinescu, Brenda Dolan, Amy P. Sullivan, Mark Hernandez, Angela M. Bosco‐Lauth, Susan C. van den Heever, Elizabeth A. Stone, Leah D. Grant, Russell Perkins, Paul J. DeMott, Sonia M. Kreidenweis

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldEngineering
TopicIcing and De-icing Technologies
Canadian institutionsnot available
FundersPacific Northwest National LaboratoryNational Centers for Environmental InformationAgricultural Research ServiceSchweizerischer Nationalfonds zur Förderung der Wissenschaftlichen ForschungBattelleRoyal Canadian Geographical SocietyColorado State UniversityU.S. Department of AgricultureNational Science Foundation
KeywordsIce nucleusEnvironmental scienceAtmospheric sciencesNucleationPhysical geographyGeologyGeographyPhysics

Abstract

fetched live from OpenAlex

Ice-nucleating particles (INPs) play a key role in ice formation and cloud microphysics and thus significantly impact the water cycle and the climate. However, our understanding of atmospheric INPs, particularly their sources, emissions, and spatiotemporal variability, is incomplete. While the enhancement of atmospheric INP concentrations with rainfall has been previously shown, a mechanistic understanding of the process is lacking. Here, we link detailed precipitation observations with near-surface atmospheric INP concentrations at a semi-arid grassland site in Colorado. Considering the during-precipitation air samples, INP concentrations positively correlate with cumulative rainfall kinetic energy and amount, suggesting that INP aerosolization is induced by raindrop and hailstone impact. By additionally analyzing the INP content of precipitation water, terrestrial source samples, and heat-treated samples, we demonstrate that local plants are the most important source of precipitation-induced INPs. Should INPs aerosolized by precipitation rise to cloud height, they could influence cloud ice fraction and initiate precipitation resulting in an aerosol-cloud-precipitation feedback.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.649
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.247
Teacher spread0.235 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2024
Admission routes1
Has abstractyes

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