MétaCan
Menu
Back to cohort
Record W4403292969 · doi:10.1002/macp.202400277

Toward In Vitro Vascular Wall Models: Digital Light Processing of Acrylate‐Endcapped Urethane‐Based Polymers into Tubular Constructs

2024· article· en· W4403292969 on OpenAlexaff
Nele Pien, Ianina Pokholenko, Nicolas Deroose, Charlotte Perneel, Rafaelle Vinturelle, Marguerite Meeremans, Diego Mantovani, Sandra Van Vlierberghe, Catharina De Schauwer

Bibliographic record

VenueMacromolecular Chemistry and Physics · 2024
Typearticle
Languageen
FieldMaterials Science
TopicElectrospun Nanofibers in Biomedical Applications
Canadian institutionsUniversité Laval
Fundersnot available
KeywordsAcrylatePolymer chemistryPolymerPolymer scienceMaterials scienceCopolymerComposite material

Abstract

fetched live from OpenAlex

Abstract Digital light processing (DLP) is emerging as a powerful tool for fabricating tissue engineering (TE) scaffolds, particularly for vascular TE and the development of representative in vitro vascular wall models. For the latter, biomaterials should mimick the biological and mechanical properties of native blood vessels. To fabricate tubular constructs, the DLP‐printing process is optimized by exploiting acrylate‐endcapped urethane‐based (AUP) polymers as the presence of the acrylate end groups render them suitable for DLP printing and desirable mechanical properties arise from the urethane segments. Four AUP variants are synthesized, exploring polyethylene glycol (PEG) and polypropylene glycol (PPG) backbones with varying acrylate functionalities (di‐acrylate versus hexa‐acrylate), namely UPEG2, UPEG6, UPPG2, and UPPG6. Tubular constructs with precise dimensions and morphology are fabricated. PPG‐based AUP polymers exhibit superior computer‐aided design/manufacturing (CAD/CAM) mimicry compared to PEG‐based derivatives. Construct characterization reveals tunable mechanical properties, with elastic moduli ranging from 45 to 259 kPa, reaching values of the human blood vessels. In particular, UPPG6 shows a two‐fold higher elastic modulus compared to UPPG2. All materials show excellent biocompatibility. Additionally, surface modification with gelatin‐methacryloyl (GELMA) significantly enhances the cytocompatibility of UPPG2 scaffolds. This study demonstrates the feasibility of fabricating tubular constructs with tunable properties using DLP and AUP polymers.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.109
Threshold uncertainty score0.937

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.222
Teacher spread0.215 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes1
Has abstractyes

Explore more

Same venueMacromolecular Chemistry and PhysicsSame topicElectrospun Nanofibers in Biomedical ApplicationsFrench-language works237,207