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Record W4403491548 · doi:10.1002/cjce.25522

Functionalization of cellulose pentamine as a promising nano‐amorphous sorbent for Zr( <scp>IV</scp> ) and Hf( <scp>IV</scp> ) ions recovery

2024· article· en· W4403491548 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

venuePublished in a venue whose home country is Canada.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2024
Typearticle
Languageen
FieldEngineering
TopicExtraction and Separation Processes
Canadian institutionsnot available
Fundersnot available
KeywordsCelluloseSurface modificationSorbentIonChemistryAmorphous solidChemical engineeringMaterials scienceOrganic chemistryAdsorption

Abstract

fetched live from OpenAlex

Abstract Due to the rising worldwide need for commercial zirconium and hafnium metals, various research studies have been conducted to investigate their extraction from ores and recovery from other waste products. By chorinating cellulose and then aminating it with tetraethylene pentamine, a cellulose‐tetraethylene pentamine (Cell‐TEPA) nanosorbent was synthesized, which resulted in active groups responsible for binding processes with the appropriate metal ions using a straightforward approach. The composition, chemical characteristics, and physical attributes of the Cell‐TEPA nanosorbent were comprehensively examined using a range of equipment, such as X‐ray diffraction (XRD), scanning electron microscope–energy dispersive X‐ray analysis (SEM–EDX), Fourier‐transform infrared spectroscopy (FT‐IR), Brunauer–Emmett–Teller (BET), and thermal gravimetric analysis (TGA). When bound to the Cell‐TEPA nanosorbent, Zr(IV) and Hf(IV) exhibited the highest absorption capacities of 70.4 and 38.2 mg/g, respectively. The most favourable sorption conditions were achieved with a feed solution pH of 1.5, a stirring period of 45 min, a metal ion concentration of 100 mg/L, and room temperature (25 ± 2°C). The adsorption data were consistent with both the Langmuir isothermal model and the pseudo‐2nd‐order reaction model. The Cell‐TEPA nanosorbent effectively extracted zirconium and hafnium ions from leach liquors derived from Wadi Rahba ore sample and Abu Khashaba concentrate sample, demonstrating their potential for future applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.108
Threshold uncertainty score0.701

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.206
Teacher spread0.196 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it