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Record W4403584954 · doi:10.1002/ppsc.202400147

Corn Stover Lignin as a Solid Acid Catalyst for the Esterification of Oleic Acid

2024· article· en· W4403584954 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueParticle & Particle Systems Characterization · 2024
Typearticle
Languageen
FieldEngineering
TopicLignin and Wood Chemistry
Canadian institutionsConcordia University
FundersConcordia UniversityNatural Sciences and Engineering Research Council of CanadaMcGill University
KeywordsCorn stoverLigninOleic acidCatalysisSolid acidChemistryOrganic chemistryStoverPulp and paper industryAgronomyBiochemistryHydrolysisBiologyCrop

Abstract

fetched live from OpenAlex

Abstract The catastrophic ramifications of fossil fuels on the environment have prompted the search for renewable energy sources. Over the recent decades, biodiesel has garnered attention as a promising direct alternative to diesel fuel; however, reliance on homogeneous catalysts and the requirement for refined vegetable oil feedstocks present financial and sustainability concerns. Thus, there exists a need for the development of sustainable and cost‐effective catalytic solutions. Herein, the application of lignin, an abundant and renewable biomass, as an effective heterogeneous catalyst is reported for biodiesel production via the esterification of oleic acid. Lignin is extracted from corn straw using sulfuric acid, which endows sulfonic acid groups (0.85 mmol g −1 ) to its structure allowing it to act as an acid catalyst without additional post‐treatments. Conversion of oleic oil to biodiesel is achieved at 97% using a 1:3 oleic acid to methanol molar ratio with a 5 wt.% catalyst loading at 90 °C after only 30 min. Moreover, the catalyst exhibits a remarkable turnover frequency of 2.61 min −1 proving its efficiency. These findings demonstrate that heterogeneous catalysts can be prepared from biomass waste offering a significantly cheaper and less intensive synthesis process and allowing for a paradigm shift to non‐edible and waste cooking oils.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.230
Threshold uncertainty score0.554

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.242
Teacher spread0.227 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it