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Record W4403862259 · doi:10.1021/acs.iecr.4c02154

Continuous Production of Resolidified Cellulose-Based Films

2024· article· en· W4403862259 on OpenAlexafffund
Yiwei Jiang, Mohammadhadi Moradian, Oana M. Nutu, Seyed Mohammad Amin Ojagh, Theo G. M. van de Ven

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2024
Typearticle
Languageen
FieldMaterials Science
TopicAdvanced Cellulose Research Studies
Canadian institutionsMcGill University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsCelluloseProduction (economics)Materials scienceChemistryEnvironmental scienceOrganic chemistryEconomics

Abstract

fetched live from OpenAlex

Films commonly used in food packaging are often derived from petroleum-based plastics, which pose a threat to the environment due to them being nonbiodegradable and nonecological. Herein, we present an approach wherein robust and flexible cellulose-based films were continuously generated using a flow casting method, involving the extrusion of dope through a slit, followed by resolidification in acid. The extruded films were deposited on a conveyor belt submerged in an acid bath and capable of operating at speeds up to 7 cm/s. The morphological and physiochemical properties of films were assessed using field emission scanning electron microscopy, solid-state 13 C NMR, and X-ray diffraction (XRD). XRD analysis revealed that carboxymethylated cellulose films regenerated at higher extrusion speeds exhibited a higher alignment in the orientation of cellulose crystals. The tensile stress of the film increased from 105 to 125 MPa as the speed of the conveyor belt increased from 0.8 to 7 cm/s. Notably, the tensile strength in the belt direction (BD) (125 MPa) is significantly higher (125 MPa) than the tensile stress in the cross direction (76 MPa). This difference confirms the anisotropic nature of the films, with cellulose chains preferentially aligning along the BD, as well as the specific crystallographic planes (11̅0) and (110).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.085
GPT teacher head0.344
Teacher spread0.259 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2024
Admission routes2
Has abstractyes

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