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Record W4403865153 · doi:10.1039/d4sc04181j

Temperature and external fields in conceptual density functional theory

2024· review· en· W4403865153 on OpenAlexafffund
Marco Franco‐Pérez, Farnaz Heidar‐Zadeh, Paul W. Ayers, Frank De Proft, Alberto Vela, José L. Gázquez, Paul Geerlings

Bibliographic record

VenueChemical Science · 2024
Typereview
Languageen
FieldChemistry
TopicChemical Thermodynamics and Molecular Structure
Canadian institutionsMcMaster UniversityQueen's University
FundersAlliance de recherche numérique du CanadaNatural Sciences and Engineering Research Council of CanadaVlaamse regeringVrije Universiteit BrusselFonds Wetenschappelijk OnderzoekCanada Research Chairs
KeywordsDensity functional theoryEpistemologyComputer scienceTheoretical physicsPsychologyStatistical physicsCognitive sciencePhysicsPhilosophyQuantum mechanics

Abstract

fetched live from OpenAlex

denotes the "field". Response functions to changes in the field can then be defined in analogy to classical thermodynamics. The electric field results display a case of a field-induced selectivity in a reaction channel of the Fukui function. Remarkably, atomic electronegativity and hardness in magnetic fields display a piecewise behavior in magnetic fields, associated to configurational jumps upon increasing field strength. The overall compression of their ranges for stronger fields may be insightful when investigating chemistry in extremely high fields. The electronegativity and hardness of diatomics under mechanical force can be traced back to changes in equilibrium distances in the neutral, cationic and anionic state, parallel with the evolution of an intrinsic atomic volume under pressure.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.716
Threshold uncertainty score0.894

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.280
Teacher spread0.264 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations16
Published2024
Admission routes2
Has abstractyes

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