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Record W4404041923 · doi:10.1021/acs.jmedchem.4c02010

A Target Class Ligandability Evaluation of WD40 Repeat-Containing Proteins

2024· article· en· W4404041923 on OpenAlexafffund
Suzanne Ackloo, Fengling Li, Magda Szewczyk, Almagul Seitova, P. Loppnau, Hong Zeng, Jin Xu, Shabbir Ahmad, Yelena A. Arnautova, Arrash J. Baghaie, Serap Beldar, Albina Bolotokova, Irene Chau, Matthew A. Clark, John W. Cuozzo, Saba Dehghani-Tafti, Jeremy S. Disch, Aiping Dong, Antoine Dumas, Jianwen A. Feng, Pegah Ghiabi, Elisa Gibson, Justin Gilmer, Brian Goldman, Stuart R. Green, Marie-Aude Guié, John P. Guilinger, Nathan Harms, Oleksandra Herasymenko, Scott Houliston, Ashley Hutchinson, Steven Kearnes, Anthony D. Keefe, Serah Kimani, Trevor J. Kramer, Maria Kutera, Haejin Angela Kwak, Cristina Lento, Yanjun Li, Jenny Liu, Joachim Loup, Raquel A. C. Machado, Christopher J. Mulhern, Sumera Perveen, Germanna Lima Righetto, Patrick Riley, Suman Shrestha, Eric A. Sigel, Madhushika Silva, Michael D. Sintchak, Belinda L. Slakman, Rhys Dylan Taylor, James Thompson, Wen Torng, Carl Underkoffler, Moritz von Rechenberg, Ryan T. Walsh, Ian R. Watson, Derek J. Wilson, Esther Wolf, Manisha Yadav, Aliakbar Khalili Yazdi, Junyi Zhang, Ying Zhang, Vijayaratnam Santhakumar, A.M. Edwards, Dalia Barsyte-Lovejoy, Matthieu Schapira, Peter J. Brown, Levon Halabelian, C.H. Arrowsmith

Bibliographic record

VenueJournal of Medicinal Chemistry · 2024
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicSignaling Pathways in Disease
Canadian institutionsPrincess Margaret Cancer CentreStructural Genomics ConsortiumYork UniversityUniversity of Toronto
FundersNational Institute of General Medical SciencesBristol-Myers Squibb CanadaGenentechInnovative Medicines InitiativeOntario Genomics InstituteUniversity of TorontoEuropean Federation of Pharmaceutical Industries and AssociationsStructural Genomics ConsortiumMerck KGaANational Institutes of HealthOntario GenomicsOffice of Research Infrastructure Programs, National Institutes of HealthGenome CanadaBayerPfizerBristol-Myers SquibbTakeda CanadaMcGill UniversityOffice of ScienceBoehringer IngelheimArgonne National LaboratoryJanssen CanadaU.S. Department of Energy
KeywordsChemistryBiochemistryClass (philosophy)Computational biologyArtificial intelligence

Abstract

fetched live from OpenAlex

Target class-focused drug discovery has a strong track record in pharmaceutical research, yet public domain data indicate that many members of protein families remain unliganded. Here we present a systematic approach to scale up the discovery and characterization of small molecule ligands for the WD40 repeat (WDR) protein family. We developed a comprehensive suite of protocols for protein production, crystallography, and biophysical, biochemical, and cellular assays. A pilot hit-finding campaign using DNA-encoded chemical library selection followed by machine learning (DEL-ML) to predict ligands from virtual libraries yielded first-in-class, drug-like ligands for 7 of the 16 WDR domains screened, thus demonstrating the broader ligandability of WDRs. This study establishes a template for evaluation of protein family wide ligandability and provides an extensive resource of WDR protein biochemical and chemical tools, knowledge, and protocols to discover potential therapeutics for this highly disease-relevant, but underexplored target class.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.003
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score0.435

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0030.002
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.311
Teacher spread0.290 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations21
Published2024
Admission routes2
Has abstractyes

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