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<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline" overflow="scroll"> <mml:msub> <mml:mi>Yb</mml:mi> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mrow> <mml:mrow> <mml:mi mathvariant="normal">O</mml:mi> </mml:mrow> </mml:mrow> <mml:mn>3</mml:mn> </mml:msub> <mml:mo>/</mml:mo> <mml:msub> <mml:mrow> <mml:mi>Mo</mml:mi> <mml:mi mathvariant="normal">O</mml:mi> </mml:mrow> <mml:mn>3</mml:mn> </mml:msub> </mml:math> connecting electrodes for tandem organic semiconductor devices

2024· article· lv· W4404090263 on OpenAlexaff
Nan Chen, Jiaxiu Man, Dongming Zhang, Dengke Wang, Juntao Hu, Changsheng Shi, Zheng‐Hong Lu

Bibliographic record

VenuePhysical Review Applied · 2024
Typearticle
Languagelv
FieldEngineering
TopicSemiconductor materials and devices
Canadian institutionsUniversity of Toronto
FundersYunnan Provincial Department of Education
KeywordsScrollAlgorithmComputer sciencePhysicsPhilosophyTheology

Abstract

fetched live from OpenAlex

This paper reports that ${\mathrm{Yb}}_{2}{\mathrm{O}}_{3}/{\mathrm{Mo}\mathrm{O}}_{3}$ stacks can be used effectively as a connecting electrode, enabling highly efficient tandem organic light-emitting diodes (OLEDs). The current efficiency of these tandem OLEDs more than doubles, from approximately 90 to 200 cd/A, compared to the single-layer devices. Additionally, this connecting electrode introduces little increase in the tandem OLED driving voltage, maintaining a value close to the sum of two single-layer devices. However, the energy-level alignments measured by ultraviolet photoemission spectroscopy show significant energy barriers in the ${\mathrm{Yb}}_{2}{\mathrm{O}}_{3}/{\mathrm{Mo}\mathrm{O}}_{3}$ stack. Analysis using photoemission measurements revealed the presence of gap states in the oxide stack and a high differential work function, 2.28 vs 6.38 eV on each side of the ${\mathrm{Yb}}_{2}{\mathrm{O}}_{3}/{\mathrm{Mo}\mathrm{O}}_{3}$ stack. Variable-temperature current-voltage measurements on ${\mathrm{Yb}}_{2}{\mathrm{O}}_{3}/{\mathrm{Mo}\mathrm{O}}_{3}$ stacks revealed that the gap states behave like Anderson-Mott localized quantum states, which form efficient hopping conduction paths for electrons and holes. These findings demonstrate that the gap states in electrodes can be effectively used to transport charges in tandem semiconductor devices.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.007
metaresearch head score (Gemma)0.005
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Scholarly communication, Open science, Research integrity, Insufficient payload (model declined to judge)
Consensus categoriesMeta-epidemiology (narrow), Science and technology studies, Research integrity, Insufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.869
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0070.005
Meta-epidemiology (narrow)0.0040.008
Meta-epidemiology (broad)0.0020.007
Bibliometrics0.0020.005
Science and technology studies0.0050.004
Scholarly communication0.0070.006
Open science0.0080.006
Research integrity0.0070.007
Insufficient payload (model declined to judge)0.6980.008

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.247
Teacher spread0.229 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2024
Admission routes1
Has abstractyes

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