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Record W4404098721 · doi:10.1016/j.epsl.2024.119094

Magmatic N2 degassing dominates nitrogen loss during sediment subduction and granitoid genesis

2024· article· en· W4404098721 on OpenAlexaff
Yunzhe Chen, Peng Wu, Tiago Valim Angelo, Christopher S. Spencer, Long Li

Bibliographic record

VenueEarth and Planetary Science Letters · 2024
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicGeochemistry and Elemental Analysis
Canadian institutionsQueen's UniversityUniversity of Alberta
Fundersnot available
KeywordsGeologySubductionGeochemistryNitrogenSedimentEarth sciencePetrologyGeomorphologyTectonicsSeismology

Abstract

fetched live from OpenAlex

• Sediment-derived granitoids are surprisingly N-poor. • N loss during granitoid genesis is mainly through magmatic N 2 degassing. • N isotopes of sediment-derived granitoids can serve for source tracing. • Water content may control N retention in granitoids. Subducting sediments contain much more abundant nitrogen (N) than the other slab components. The fate of sedimentary N along subduction directly determines the quantity of surficial N that can be released back to the atmosphere/crust or further delivered to the deep mantle, which has a strong impact on the long-term evolution of the N budgets and isotopic signatures of Earth's major reservoirs. Previous studies on the fate of subducted sedimentary N have been intensively focused on assessing the extent of metamorphic N devolatilization from metasedimentary rocks varying from ultrahigh-pressure eclogites facies (subducted to as deep as 90 km) in cold subduction zones to medium-pressure amphibolite facies in extremely hot subduction zones. However, the fate of sedimentary N after these metamorphic stages, particularly during sediment melting and subsequent magmatic crystallization, has not been examined so far. Here, we present the N data of the Cretaceous peraluminous granitoids in the Oman-United Arab Emirates area, which were formed by melting of subducted pelagic sediments followed by intrusion and crystallization in the lithospheric mantle before the entire lithospheric section was obducted to form the Oman-United Arab Emirates ophiolites. The 27 studied samples show surprisingly low N contents (4.0 - 13.7 ppm; mean: 6.9 ± 2.3 ppm; 1σ) and a narrow δ 15 N range (mostly in the range of –1.4‰ to +2.2‰; mean: +0.4 ± 1.5‰; 1σ). Data modeling indicates that the N in these granitoids contains little mantle contribution and was predominantly inherited from their source rocks. Compared with potential source rocks, these granitoids display orders of magnitude lower N contents but comparable δ 15 N values, indicating that the significant N loss during the genesis of these granitoids was associated with little N isotope fractionation. This suggests that magmatic N 2 degassing (with minor N isotope fractionation) rather than metamorphic N devolatilization (with much larger N isotope fractionation) is the dominant mechanism driving the N loss from subducted sediments.

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How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.032
Threshold uncertainty score0.683

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.168
Teacher spread0.164 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2024
Admission routes1
Has abstractyes

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