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Record W4404290419 · doi:10.1016/j.clema.2024.100278

Effects of the surface properties and particle size of hydrated lime on desulfurization

2024· article· en· W4404290419 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueCleaner Materials · 2024
Typearticle
Languageen
FieldEngineering
TopicIndustrial Gas Emission Control
Canadian institutionsGraymont (Canada)Cégep de JonquièreUniversité du Québec à Chicoutimi
Fundersnot available
KeywordsFlue-gas desulfurizationLimeParticle sizeParticle (ecology)Materials scienceChemical engineeringMineralogyMetallurgyChemistryGeologyOrganic chemistryEngineering

Abstract

fetched live from OpenAlex

In the gas treatment center in smelters, hydrogen fluoride (HF) is separated from the outlet gases of electrolysis cells, which are used to produce aluminum from alumina. However, SO 2 largely remains in the effluent gas. Another method has to be developed to separate this gas which is harmful to the environment. In this study, semi-dry desulfurization of a SO 2 containing gas was performed at low SO 2 concentrations using hydrated lime [Ca(OH) 2 ] as a catalytic desulfurizer under specific humidity conditions. The low reaction temperature of 100 °C and minimal use of the Ca-based desulfurizer under 17 % relative humidity achieved more than 95 % removal of SO 2 . The morphological changes and presence of sulfur in different lime samples were analyzed by scanning electron microscopy and energy-dispersive X-ray spectroscopy. Brunauer–Emmett–Teller (BET) analysis showed changes in the surface properties of hydrated lime after desulfurization. X-ray photoelectron spectroscopy (XPS) analysis provided the phase and composition identification of the sulfur species on hydrated lime and the CaSO 3 /CaSO 4 product ratio. Based on the experimental results, the optimum catalyst surface area with a specific particle size is critical to the effective conversion of Ca(OH) 2 into CaSO 3 and CaSO 4 . The practicality of a Ca-based desulfurizer and its ability to convert into the required product may be the key to reducing the overall cost of desulfurization in aluminum industry.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.188

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.186
Teacher spread0.174 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it