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Advanced functional membranes based on amphiphilic copolymers

2024· article· en· W4404323875 on OpenAlexafffund
Zhuan Yi, Lijing Zhu, Ruiyan Xiong, Chuanjie Fang, Bao‐Ku Zhu, Hongbo Zeng

Bibliographic record

VenueProgress in Polymer Science · 2024
Typearticle
Languageen
FieldEngineering
TopicFuel Cells and Related Materials
Canadian institutionsUniversity of Alberta
FundersNational Key Research and Development Program of ChinaNational Natural Science Foundation of ChinaKey Technologies Research and Development ProgramZhejiang UniversityKey Research and Development Program of Zhejiang ProvinceNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsCopolymerAmphiphileMembraneMaterials sciencePolymer sciencePolymer chemistryNanotechnologyChemical engineeringChemistryPolymerEngineeringComposite material

Abstract

fetched live from OpenAlex

Membranes with advanced and novel functions play important roles in emerging applications ranging from industrial separations, water purification , energy harvesting and storage, healthcare, biomimetic membranes and more. The performance of membranes in these critical applications is fundamentally determined by their interfacial interactions with surrounding ions, molecules, particles, emulsions, and bioactive agents . Amphiphilic copolymers containing both hydrophobic and hydrophilic segments will spontaneously assemble into multiphase and hierarchical structures, providing a general solution for regulating the surface physicochemical properties of membranes used in the aforementioned urgent applications. Controlled synthesis of amphiphilic copolymers and the methods for fabricating membranes from these copolymers with predetermined performance are fundamentally important for their applications. In this work, we first summarize the polymerization techniques for synthesizing amphiphilic copolymers used for membrane materials. We then review the methods for fabricating membranes from amphiphilic copolymers and highlight the urgent applications of advanced functional membranes derived from them. We also discuss some remaining challenges and provide insights into future directions, especially as the circular polymer economy and artificial intelligence are setting new requirements for polymer science . This work offers a comprehensive overview of recent advances in functional materials based on amphiphilic polymers, including the working principles and relationships between polymer structure , processing strategies, and membrane performance , which provides new insights into the development of high-performance and next-generation polymeric membranes through the precise, functionality-driven synthesis of novel amphiphilic copolymers and the controlled fabrication of membranes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.002
Open science0.0000.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.231
Teacher spread0.224 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations21
Published2024
Admission routes2
Has abstractyes

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