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Record W4404523769 · doi:10.1016/j.cej.2024.157824

Bio-inspired magnetically induced self-assembling Janus solar evaporator with antifouling and antiscaling properties

2024· article· en· W4404523769 on OpenAlexfundno aff
Pan Huang, Charley Huang, Yongxiang Sun, Ziqian Zhao, Lin Yang, H.P. Yang, Lu Gong, Wenshuai Yang, Hongbo Zeng

Bibliographic record

VenueChemical Engineering Journal · 2024
Typearticle
Languageen
FieldEnergy
TopicSolar-Powered Water Purification Methods
Canadian institutionsnot available
FundersNatural Sciences and Engineering Research Council of CanadaCanada Foundation for Innovation
KeywordsJanusBiofoulingNanotechnologyMaterials scienceChemistryMembrane

Abstract

fetched live from OpenAlex

• A magnetically induced self-assembling Janus solar evaporator was fabricated. • The anisotropic evaporator achieved an evaporation rate of 2.13 kg m −2 h −1 . • The PFDTES modification imparts the photothermal layer with antifouling properties. • Interactions in the evaporator and antifouling properties were probed by AFM. Engineering solar evaporators with Janus structures is crucial for facilitating water transition and heat localization to enhance water evaporation efficiency. However, the fragile discontinuous bilayer structures and unavoidable surface fouling significantly hinder their application. Herein, inspired by the Janus structure of Black Amanita mushrooms, we designed a robust solar evaporator with an integrated wood-like and Janus structure using directional freeze-casting and magnetically induced self-assembly of polypyrrole-coated Fe 3 O 4 particles as a build-in photothermal top layer within a hydrophilic matrix, followed by covering it with an additional hydrophobic fluorine layer to simultaneously regulate surface wettability and antifouling properties. Incorporating the hydrophobic fluorine layer onto the solar evaporator not only enhances its water evaporation efficiency via thermal localization effects, but also prevents fouling, salt, and dust scaling accumulation on its surface, facilitating water transportation, thus achieving a groundbreaking performance with the evaporation rate of 2.13 kg m −2 h −1 under one sun irradiation. Moreover, the mechanical performance of the as-prepared solar evaporator can be further optimized by precisely modulating supramolecular interactions within its structure, achieving Young’s modulus over 4 MPa and maintaining structural integrity after the peel-off tests. The fabricated solar evaporator enables highly efficient water purification from artificial seawater, oil-in-water emulsions, and industrial wastewater, providing a rational strategy for designing high-yield solar evaporation systems for wastewater containing complex contaminants.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.000
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.230
Teacher spread0.213 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations15
Published2024
Admission routes1
Has abstractyes

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