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Record W4404564437 · doi:10.1016/j.jece.2024.114885

Understanding the physicochemical structure of biochar affected by feedstock, pyrolysis conditions, and post-pyrolysis modification methods – A meta-analysis

2024· article· en· W4404564437 on OpenAlexaff
Mohammad Ghorbani, Elnaz Amirahmadi, Wim Cornelis, Khaled Zoroufchi Benis

Bibliographic record

VenueJournal of environmental chemical engineering · 2024
Typearticle
Languageen
FieldEngineering
TopicThermochemical Biomass Conversion Processes
Canadian institutionsDalhousie University
Fundersnot available
KeywordsBiocharPyrolysisRaw materialChemistryPulp and paper industrySurface modificationChemical engineeringWaste managementMaterials scienceOrganic chemistryEngineering

Abstract

fetched live from OpenAlex

The impact of feedstock type, pyrolysis conditions, and post-pyrolysis modifications on the physicochemical properties of biochar has not been systematically evaluated. To this, a comprehensive meta-analysis was conducted to assess the impact of 17 effective variables including three groups of modification techniques (acidic, alkalic, H 2 O 2 , metal oxides , microbial, organic acids, physical, soil mineral), pyrolysis temperature (<400, 400–550, >550 °C), and feedstocks (herbaceous, hull, manure, nut, straw, wood). Also, 26 properties of the biochar were identified as being impacted; some of the most important among them are pH, cation exchange capacity (CEC), ash content (AC), specific surface area (SSA), carbonization (H/C), and surface functional groups (SFGs). The CEC of biochar modified by acidic, and soil mineral treatment significantly increased by 44.8 % and 48.5 %. The H/C ratio of biochar decreased in alkalic modification with a negative effect size of 7.2 %. Soil minerals, metal oxides, and alkalic modifications resulted in a positive change in AC with a 20.9 %, 15.7 %, and 13.6 % increase. Also, the highest SSA of modified biochar was observed when acidic and H 2 O 2 modification methods were applied, with 57.1 % and 53.4 % effect sizes. Further, high pyrolysis temperature (>550 °C) aided in significantly increasing SSA and SFGs on modified biochar. Overall, the strong association of acidic modifiers, high pyrolysis temperature, and high lignin-based feedstock could contribute to high SSA, SFGs, and absorption efficiency of biochar. This meta-analysis establishes a robust comparative framework, advancing the precision of biochar modification strategies to maximize physicochemical properties for improved environmental remediation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.048
Threshold uncertainty score0.765

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.243
Teacher spread0.222 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations28
Published2024
Admission routes1
Has abstractyes

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