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Optimizing hydrogen-rich gas production by steam gasification with integrated CaO-based adsorbent materials for CO2 capture: Machine learning approach

2024· article· en· W4404588564 on OpenAlexafffund
Mohammad Rahimi, Shakirudeen A. Salaudeen

Bibliographic record

VenueInternational Journal of Hydrogen Energy · 2024
Typearticle
Languageen
FieldEngineering
TopicChemical Looping and Thermochemical Processes
Canadian institutionsMcMaster University
FundersNatural Sciences and Engineering Research Council of CanadaOntario Ministry of Natural Resources and Forestry
KeywordsHydrogen productionSteam reformingProcess engineeringAdsorptionHydrogenSyngasProduction (economics)Materials scienceChemical engineeringEnvironmental scienceChemistryEngineeringPhysical chemistry

Abstract

fetched live from OpenAlex

The sorption-enhanced steam gasification of biomass with an integrated carbon dioxide (CO 2 ) capture is a promising process for hydrogen production. By using machine learning (ML) approaches to reduce the amount of CO 2 , this study aimed for prediction and optimization of gaseous products with a higher concentration of hydrogen. ML schemes are applied to hydrogen-rich syngas produced through calcium oxide-based adsorbent. Four predictive techniques are applied on the intrinsic constituents of biomass, adsorbents properties, steam gasification ratio, and temperature to predict the concentrations of hydrogen and CO 2 . The accuracies of ML models demonstrated high feasibility of ML to predict the hydrogen and CO 2 with R-squared (R 2 ) of 0.92; and 6.77 to 7.44 vol% of root-mean-square error (RMSE), respectively. Support vector machine (SVM) is optimized by tuning training data size and radial basis kernel ( rbf ) function. Also, the single and multi-objective(s) genetic algorithm approaches optimized the value of hydrogen concentration by Max f max ( H 2 ) by ∼84 and 88 vol%, respectively. Sensitivity analysis showed the fixed carbon/volatile matter, oxygen content, adsorbent/steam to biomass ratios, and gasification temperature in the range of 7–20 vol% of mean absolute percentage error (MAPE) on hydrogen content. The optimized input sets for the ML modelling procedure improved the hydrogen concentration by within 5 vol%. The results indicate a high proficiency of the ML models in accurate prediction of hydrogen gas in the gasification process. • Sorption-enhanced steam gasification of biomass evaluated by ML models. • ML models KNN, SVM, RF, and DT are used to predict hydrogen and CO 2 concentrations. • SVM and RF exhibited 0.91 to 0.92 of R 2 ; and 6.77 to 7.44 vol% of RMSEs. • Sensitivity analysis and genetic algorithm maximize hydrogen concentration by CO 2 reduction.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.122
Threshold uncertainty score0.681

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.212
Teacher spread0.204 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations13
Published2024
Admission routes2
Has abstractyes

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