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Record W4404624951 · doi:10.1016/j.jechem.2024.11.018

Exploring properties of hyperbranched polymers in anion exchange membranes for fuel cells and its potential integration for water electrolysis: A review

2024· review· en· W4404624951 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueJournal of Energy Chemistry · 2024
Typereview
Languageen
FieldEngineering
TopicFuel Cells and Related Materials
Canadian institutionsUniversité du Québec à Trois-Rivières
Fundersnot available
KeywordsElectrolysisFuel cellsMembranePolymerIon exchangeMaterials scienceChemical engineeringIon-exchange membranesIonChemistryNanotechnologyElectrodeOrganic chemistryComposite materialEngineeringBiochemistryPhysical chemistry

Abstract

fetched live from OpenAlex

The graphical abstract highlights the hyperbranched anion exchange membranes with linear, dendritic, and terminal units for efficient hydrogen production in water electrolysis. Anion-exchange membrane water electrolysers (AEMWEs) and fuel cells (AEMFCs) are critical technologies for converting renewable resources into green hydrogen (H 2 ), where anion-exchange membranes (AEMs) play a vital role in efficiently transporting hydroxide ions (OH − ) and minimizing fuel crossover, thus enhancing overall efficiency. While conventional AEMs with linear, side-chain, and block polymer architectures show promise through functionalization, their long-term performance remains a concern. To address this, hyperbranched polymers offer a promising alternative due to their three-dimensional structure, higher terminal functionality, and ease of functionalization. This unique architecture provides interconnected ion transport pathways, fractional free volume, and enhanced long-term stability in alkaline environments. Recent studies have achieved conductivities as high as 304.5 mS cm −1 , attributed to their improved fractional free volume and microphase separation in hyperbranched AEMs. This review explores the chemical, mechanical, and ionic properties of hyperbranched AEMs in AEMFCs and assesses their potential for application in AEMWEs. Strategies such as blending and structural functionalisation have significantly improved the properties by promoting microphase separation and increasing the density of cationic groups on the polymer surface. The review provides essential insights for future research, highlighting the challenges and opportunities in developing high-performance hyperbranched AEMs to advance hydrogen energy infrastructure.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.576
Threshold uncertainty score0.705

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.047
GPT teacher head0.237
Teacher spread0.190 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it