MétaCan
Menu
Back to cohort
Record W4404630346 · doi:10.1016/j.colsuc.2024.100051

A zwitterionic surfactant concentrates sulfolane in floating foams, to purify water

2024· article· en· W4404630346 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueColloids and Surfaces C Environmental Aspects · 2024
Typearticle
Languageen
FieldChemistry
TopicSurfactants and Colloidal Systems
Canadian institutionsUniversity of Guelph
FundersNatural Sciences and Engineering Research Council of CanadaShell Canada
KeywordsSulfolanePulmonary surfactantChemistryChromatographyChemical engineeringMaterials scienceOrganic chemistryEngineeringBiochemistry

Abstract

fetched live from OpenAlex

Sulfolane is a worldwide groundwater miscible pollutant, used for carbon capture and sour gas treatment. It is heavier than water and can sink when spilled in low salinity aquifers, posing remedial challenges. There are no strategies to prevent sulfolane plunging, other than pumping large groundwater volumes. We show that the zwitterionic surfactant cocamidopropyl betaine (CAPB) interacts with sulfolane, producing a stable floating foam, in which sulfolane is concentrated by >140 %. The foam forms by bubbling air or mild mixing. CAPB is surface active in either water or in aqueous sulfolane mixtures, and its films stabilize the air-water interface even upon significant deformation. CAPB-sulfolane interactions disrupt the water network, thereby decreasing the heat and onset of water evaporation from the foam. While CAPB successfully concentrated sulfolane, Tween 20 did not. Cationic cetyltrimethylammonium bromide binds sulfolane, but extraction of sulfolane was not possible due to foam instability. • Sulfolane is a worldwide groundwater miscible pollutant. • Sulfolane is heavier than water and plunges, with risks to low-salinity aquifers. • Cocoamidopropyl betaine (CAPB) stabilizes foam in aqueous sulfolane solutions. • CAPB concentrates sulfolane in the floating foam by >140 %, cleaning water. • Water vaporization is promoted from foams containing water+sulfolane+CAPB.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.068
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.196
Teacher spread0.191 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it